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Lattice Opening Upon Bulk Reductive Covalent Functionalization of Black Phosphorus

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Lattice Opening Upon Bulk Reductive Covalent Functionalization of Black Phosphorus

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dc.contributor.author Wild, Stefan es_ES
dc.contributor.author Fickert, Michael es_ES
dc.contributor.author Mitrovic, Aleksandra es_ES
dc.contributor.author Lloret, Vicent es_ES
dc.contributor.author Neiss, Christian es_ES
dc.contributor.author Vidal Moya, José Alejandro es_ES
dc.contributor.author Rivero-Crespo, Miguel Ángel es_ES
dc.contributor.author Leyva Perez, Antonio es_ES
dc.contributor.author Werbach, Katharina es_ES
dc.contributor.author Peterlik, Herwig es_ES
dc.contributor.author Grabau, Mathias es_ES
dc.contributor.author Wittkamper, Haiko es_ES
dc.contributor.author Papp, Christian es_ES
dc.contributor.author Steinrück, Hans-Peter es_ES
dc.contributor.author Pichler, Thomas es_ES
dc.contributor.author Gorling, Andreas es_ES
dc.date.accessioned 2023-05-18T18:00:13Z
dc.date.available 2023-05-18T18:00:13Z
dc.date.issued 2019-04-16 es_ES
dc.identifier.issn 1433-7851 es_ES
dc.identifier.uri http://hdl.handle.net/10251/193466
dc.description This is the peer reviewed version of the following article: Wild, S., Fickert, M., Mitrovic, A., Lloret, V., Neiss, C., Vidal¿Moya, J. A., ... & Hirsch, A. (2019). Lattice opening upon bulk reductive covalent functionalization of black phosphorus. Angewandte Chemie International Edition, 58(17), 5763-5768, which has been published in final form at https://doi.org/10.1002/anie.201811181. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Self-Archiving." es_ES
dc.description.abstract [EN] The chemical bulk reductive covalent functionalization of thin-layer black phosphorus (BP) using BP intercalation compounds has been developed. Through effective reductive activation, covalent functionalization of the charged BP by reaction with organic alkyl halides is achieved. Functionalization was extensively demonstrated by means of several spectroscopic techniques and DFT calculations; the products showed higher functionalization degrees than those obtained by neutral routes. es_ES
dc.description.sponsorship A.H. and G.A. acknowledge the European Research Council (ERC Advanced Grant 742145 B-PhosphoChem to A.H., and ERC Starting Grant 2D-PnictoChem 804110 to G.A.) for support. The research leading to these results was partially funded by the European Union Seventh Framework Programme under grant agreement No. 604391 Graphene Flagship. G.A. has received financial support through the Postdoctoral Junior Leader Fellowship Programme from "la Caixa" Banking Foundation (LCF/BQ/PI18/11630018). G.A. thanks the Deutsche Forschungsgemeinschaft (DFG; FLAG-ERA AB694/2-1), the Generalitat Valenciana (SEJI/2018/034 grant), and the FAU (Emerging Talents Initiative grant #WS16-17_Nat_04) for support. A.H. and A.G. thank the SFB 953 "Synthetic Carbon Allotropes" funded by the DFG for support and the Cluster of Excellence "Engineering of Advanced Materials". A.G. is grateful for funding from the Free State of Bavaria (Research Network "Solar Technologies go Hybrid"). A.M. thanks the Alexander von Humboldt (AvH) Foundation for a postdoctoral fellowship. This work was supported by the MINECO (Spain) through the Excellence Unit Maria de Maeztu (MDM-2015-0538) and the Project CTQ2017-86735-P. es_ES
dc.language Inglés es_ES
dc.publisher John Wiley & Sons es_ES
dc.relation.ispartof Angewandte Chemie International Edition es_ES
dc.rights Reconocimiento - No comercial - Sin obra derivada (by-nc-nd) es_ES
dc.title Lattice Opening Upon Bulk Reductive Covalent Functionalization of Black Phosphorus es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1002/anie.201811181 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/CTQ2017-86735-P/ES/CATALISIS CON ATOMOS METALICOS AISLADOS Y CLUSTERES ULTRAPEQUEÑOS BIEN DEFINIDOS, SIN LIGANDOS Y CONFINADOS/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/DFG//FLAG-ERA AB694%2F2-1/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/EC/FP7/604391/EU es_ES
dc.relation.projectID info:eu-repo/grantAgreement/DFG//SFB 953 / es_ES
dc.relation.projectID info:eu-repo/grantAgreement/EC/H2020/742145/EU es_ES
dc.relation.projectID info:eu-repo/grantAgreement/GVA//SEJI%2F2018%2F034/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/EC/H2020/804110/EU es_ES
dc.relation.projectID info:eu-repo/grantAgreement/Fundació Bancària Caixa d'Estalvis i Pensions de Barcelona//11630018/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//MDM-2015-0538/ES/INSTITUTO DE CIENCIA MOLECULAR/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/FAU//WS16-17_Nat_04/ es_ES
dc.rights.accessRights Abierto es_ES
dc.description.bibliographicCitation Wild, S.; Fickert, M.; Mitrovic, A.; Lloret, V.; Neiss, C.; Vidal Moya, JA.; Rivero-Crespo, MÁ.... (2019). Lattice Opening Upon Bulk Reductive Covalent Functionalization of Black Phosphorus. Angewandte Chemie International Edition. 58(17):5763-5768. https://doi.org/10.1002/anie.201811181 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1002/anie.201811181 es_ES
dc.description.upvformatpinicio 5763 es_ES
dc.description.upvformatpfin 5768 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 58 es_ES
dc.description.issue 17 es_ES
dc.identifier.pmid 30675972 es_ES
dc.identifier.pmcid PMC7318246 es_ES
dc.relation.pasarela S\383596 es_ES
dc.contributor.funder European Commission es_ES
dc.contributor.funder Generalitat Valenciana es_ES
dc.contributor.funder Deutsche Forschungsgemeinschaft es_ES
dc.contributor.funder Agencia Estatal de Investigación es_ES
dc.contributor.funder Alexander von Humboldt Foundation es_ES
dc.contributor.funder Ministerio de Economía y Competitividad es_ES
dc.contributor.funder Friedrich-Alexander-Universität Erlangen-Nürnberg es_ES
dc.contributor.funder Bayerisches Staatsministerium für Wissenschaft und Kunst es_ES
dc.contributor.funder Fundació Bancària Caixa d'Estalvis i Pensions de Barcelona es_ES


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