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dc.contributor.author | Li, Yubing | es_ES |
dc.contributor.author | Zeng, Lei | es_ES |
dc.contributor.author | Pang, Ge | es_ES |
dc.contributor.author | Wei, Xueer | es_ES |
dc.contributor.author | Wang, Mengheng | es_ES |
dc.contributor.author | Cheng, Kang | es_ES |
dc.contributor.author | Kang, Jincan | es_ES |
dc.contributor.author | Serra Alfaro, José Manuel | es_ES |
dc.contributor.author | Zhang, Qinghong | es_ES |
dc.contributor.author | Wang, Ye | es_ES |
dc.date.accessioned | 2024-04-16T18:02:37Z | |
dc.date.available | 2024-04-16T18:02:37Z | |
dc.date.issued | 2023-05-05 | es_ES |
dc.identifier.issn | 0926-3373 | es_ES |
dc.identifier.uri | http://hdl.handle.net/10251/203534 | |
dc.description.abstract | [EN] The chemical conversion of CO2 into hydrocarbon fuels and chemicals using green hydrogen not only utilizes abundant CO2 as a carbon feedstock but also enables the storage of hydrogen. Herein, we investigate the direct hydrogenation of CO2 to gasoline and olefins over a series of bifunctional iron-zeolite tandem catalysts operated at high temperatures (> 300 degrees C). This process may efficiently utilize CO2 discharged from industrial combustion and green H2 produced by solid oxide electrolytic cells (SOEC). The optimized FeMnK+H-ZSM-5 catalyst offers a 70% selectivity of C5-C11 range hydrocarbons together with a 17% selectivity of C2-C4 lower olefins at 320 degrees C. The CO2 conversion levels and the aromatics contents could be greatly enhanced as the temperature increases from 320 degrees C to 400 degrees C. The hydrocarbon distribution is mainly determined by the micropore size of the zeolites. The dynamic evolution of bifunctional catalysts and its impact on bifunctional catalysis was systematically investigated. | es_ES |
dc.description.sponsorship | This work was supported by the National Key Research and Devel- opment Program of Ministry of Science and Technology (No. 2019YFE0104400) , the National Natural Science Foundation of China (Nos. 91945301, 22121001, 22222206, 22072120, and 22202165) , and the China Postdoctoral Science Foundation (No. 2021M702733) . | es_ES |
dc.language | Inglés | es_ES |
dc.publisher | Elsevier | es_ES |
dc.relation.ispartof | Applied Catalysis B Environmental | es_ES |
dc.rights | Reconocimiento - No comercial - Sin obra derivada (by-nc-nd) | es_ES |
dc.subject | Zeolite | es_ES |
dc.subject | Liquid fuels | es_ES |
dc.subject | CO2 reduction | es_ES |
dc.subject | Bifunctional | es_ES |
dc.subject | Hydrogen storage | es_ES |
dc.title | Direct conversion of carbon dioxide into liquid fuels and chemicals by coupling green hydrogen at high temperature | es_ES |
dc.type | Artículo | es_ES |
dc.identifier.doi | 10.1016/j.apcatb.2022.122299 | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/NSFC//22121001/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/NSFC//22222206/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/NSFC//22072120/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/NSFC//22202165/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/NSFC//91945301/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/NKRDPC//2019YFE0104400/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/China Postdoctoral Science Foundation//2021M702733/ | es_ES |
dc.rights.accessRights | Embargado | es_ES |
dc.date.embargoEndDate | 2024-12-31 | es_ES |
dc.description.bibliographicCitation | Li, Y.; Zeng, L.; Pang, G.; Wei, X.; Wang, M.; Cheng, K.; Kang, J.... (2023). Direct conversion of carbon dioxide into liquid fuels and chemicals by coupling green hydrogen at high temperature. Applied Catalysis B Environmental. 324. https://doi.org/10.1016/j.apcatb.2022.122299 | es_ES |
dc.description.accrualMethod | S | es_ES |
dc.relation.publisherversion | https://doi.org/10.1016/j.apcatb.2022.122299 | es_ES |
dc.type.version | info:eu-repo/semantics/publishedVersion | es_ES |
dc.description.volume | 324 | es_ES |
dc.relation.pasarela | S\510770 | es_ES |
dc.contributor.funder | China Postdoctoral Science Foundation | es_ES |
dc.contributor.funder | National Natural Science Foundation of China | es_ES |
dc.contributor.funder | National Key Research and Development Program of China | es_ES |