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Composition-dependent physical properties of poly[(vinylidene fluoride)-co-trifluoroethylene] poly(ethylene oxide) blends

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Composition-dependent physical properties of poly[(vinylidene fluoride)-co-trifluoroethylene] poly(ethylene oxide) blends

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dc.contributor.author Costa, Carlos M. es_ES
dc.contributor.author Tamano Machiavello, M.N. es_ES
dc.contributor.author Gómez Ribelles, José Luís es_ES
dc.contributor.author Lanceros Mendez, Senen es_ES
dc.date.accessioned 2016-05-17T07:29:08Z
dc.date.available 2016-05-17T07:29:08Z
dc.date.issued 2013-05
dc.identifier.issn 0022-2461
dc.identifier.uri http://hdl.handle.net/10251/64185
dc.description.abstract Polymer blends based on poly(vinylidene fluoride-co-trifluoroethylene) copolymers, P(VDF-TrFE), and poly(ethylene oxide), PEO, with varying compositions have been prepared by solvent casting. In this way, P(VDF-TrFE) crystallizes from the solution while solvent evaporates, while PEO crystallizes from the melt during cooling to room temperature. The surface morphology of the polymer blends indicates the transition from the fibrillar microstructure typical of PVDF-TrFE to the spherulite structure characteristic of PEO. The vibration mode characteristics of P(VDF-TrFE) are not influenced by the presence of PEO in the polymer blend. Confinement of PEO in the P(VDF-TrFE) phase change the conformation of PEO from trans to helix, increasing this transformation for increasing P(VDF-TrFE) content in the polymer blends. Sequential crystallization of the two polymers produce separated amorphous phases whose independent cooperative conformational motions are revealed by two main dynamic-mechanical relaxations. No chemical interaction seems to exist between the polymers within the blend. es_ES
dc.description.sponsorship This study is funded by FEDER funds through the "Programa Operacional Factores de Competitividade - COMPETE'' and by national funds by FCT-Fundacao para a Ciencia e a Tecnologia, Project References NANO/NMed-SD/0156/2007 and PTDC/CTM/69316/2006. C. M. C. also thanks the FCT for the Grant SFRH/BD/68499/2010. The authors also thank support from the COST Action MP1003, the "European Scientific Network for Artificial Muscles'' (ESNAM). JLGR acknowledges the support of the Spanish Ministry of Education through Project No. MAT2010-21611-C03-01 (including the FEDER financial support). CIBER-BBN is an initiative funded by the VI National R&D&D&i Plan 2008-2011, Iniciativa Ingenio 2010, Consolider Program, CIBER Actions and financed by the Instituto de Salud Carlos III with assistance from the European Regional Development Fund. en_EN
dc.language Inglés es_ES
dc.publisher Springer Verlag es_ES
dc.relation.ispartof Journal of Materials Science es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject PERFORMANCE ELECTROACTIVE POLYMERS es_ES
dc.subject LITHIUM-ION BATTERY es_ES
dc.subject BETA-PVDF FILMS es_ES
dc.subject POLY(ETHYLENE OXIDE) es_ES
dc.subject VINYLIDENE FLUORIDE es_ES
dc.subject THERMAL-DEGRADATION es_ES
dc.subject POLYETHYLENE OXIDE es_ES
dc.subject PHASE-TRANSITION es_ES
dc.subject SOLID-STATE es_ES
dc.subject POLY(VINYLIDENE FLUORIDE) es_ES
dc.subject.classification ORGANIZACION DE EMPRESAS es_ES
dc.subject.classification MAQUINAS Y MOTORES TERMICOS es_ES
dc.title Composition-dependent physical properties of poly[(vinylidene fluoride)-co-trifluoroethylene] poly(ethylene oxide) blends es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1007/s10853-013-7141-z
dc.relation.projectID info:eu-repo/grantAgreement/MICINN//MAT2010-21611-C03-01/ES/MATERIALES BIOESTABLES Y BIOREABSORBIBLES A LARGO PLAZO COMO SOPORTES MACROPOROSOS PARA LA REGENERACION DEL CARTILAGO ARTICULAR/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/FCT/SFRH/SFRH%2FBD%2F68499%2F2010/PT/
dc.relation.projectID info:eu-repo/grantAgreement//COST/MP1003/EU/European Scientific Network for Artificial Muscles/ESNAM/
dc.relation.projectID info:eu-repo/grantAgreement/COST//MP1003/EU/European Scientific Network for Artificial Muscles (ESNAM)/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/FCT/5876-PPCDTI/109368/PT/“Smart joint implants using bionanocomposites-(SIMBIO)”/
dc.relation.projectID info:eu-repo/grantAgreement/FCT/5876-PPCDTI/69316/PT/Multiferroic, magnetoelectric and metallic micro and nanocomposites based on electroactive polymers for advanced applications/
dc.rights.accessRights Cerrado es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Termodinámica Aplicada - Departament de Termodinàmica Aplicada es_ES
dc.description.bibliographicCitation Costa, CM.; Tamano Machiavello, M.; Gómez Ribelles, JL.; Lanceros Mendez, S. (2013). Composition-dependent physical properties of poly[(vinylidene fluoride)-co-trifluoroethylene] poly(ethylene oxide) blends. Journal of Materials Science. 48(9):3494-3504. https://doi.org/10.1007/s10853-013-7141-z es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion http://dx.doi.org/10.1007/s10853-013-7141-z es_ES
dc.description.upvformatpinicio 3494 es_ES
dc.description.upvformatpfin 3504 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 48 es_ES
dc.description.issue 9 es_ES
dc.relation.senia 260196 es_ES
dc.contributor.funder Ministerio de Ciencia e Innovación es_ES
dc.contributor.funder European Cooperation in Science and Technology es_ES
dc.contributor.funder Instituto de Salud Carlos III es_ES
dc.contributor.funder European Regional Development Fund es_ES
dc.contributor.funder Fundação para a Ciência e a Tecnologia, Portugal
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