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Study of the Effect of Inorganic Particles on the Gas Transport Properties of Glassy Polyimides for Selective CO2 and H2O Separation

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Study of the Effect of Inorganic Particles on the Gas Transport Properties of Glassy Polyimides for Selective CO2 and H2O Separation

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dc.contributor.author Escorihuela-Roca, Sara es_ES
dc.contributor.author Valero, Lucía es_ES
dc.contributor.author Tena, Alberto es_ES
dc.contributor.author Shishatskiy, Sergey es_ES
dc.contributor.author Escolástico Rozalén, Sonia es_ES
dc.contributor.author Brinkmann, Torsten es_ES
dc.contributor.author Serra Alfaro, José Manuel es_ES
dc.date.accessioned 2020-06-24T03:31:21Z
dc.date.available 2020-06-24T03:31:21Z
dc.date.issued 2018-12 es_ES
dc.identifier.uri http://hdl.handle.net/10251/146876
dc.description.abstract [EN] Three polyimides and six inorganic fillers in a form of nanometer-sized particles were studied as thick film solution cast mixed matrix membranes (MMMs) for the transport of CO2, CH4, and H2O. Gas transport properties and electron microscopy images indicate good polymer-filler compatibility for all membranes. The only filler type thatdemonstrated good distribution throughout the membrane thickness at 10 wt.% loading was BaCe0.2Zr0.7Y0.1O3 (BCZY). The influence of this filler on MMM gas transport properties was studied in detail for 6FDA-6FpDA in a filler content range from one to 20 wt.% and for Matrimid((R)) and P84((R)) at 10 wt.% loading. The most promising result was obtained for Matrimid((R))10 wt.% BCZY MMM, which showed improvement in CO2 and H2O permeabilities accompanied by increased CO2/CH4 selectivity and high water selective membrane at elevated temperatures without H2O/permanent gas selectivity loss. es_ES
dc.description.sponsorship This work was financially supported by the Spanish Government (SEV-2016-0683, SVP-2014-068356, Project ENE2014-57651-R and IJCI-2016-28330 grants) and GeneralitatValenciana (PROMETEO/2018/006 grant) and Helmholtz-Zentrum Geesthacht (HZG) through the technology transfer project program and by the Helmholtz Association of German Research Centers through the Helmholtz Portfolio MEMBRAIN. es_ES
dc.language Inglés es_ES
dc.publisher MDPI AG es_ES
dc.relation.ispartof Membranes es_ES
dc.rights Reconocimiento (by) es_ES
dc.subject Mixed matrix membranes es_ES
dc.subject Carbon dioxide es_ES
dc.subject Water vapor permeability es_ES
dc.subject Polyimides es_ES
dc.subject Inorganic fillers es_ES
dc.subject Gas separation membranes es_ES
dc.subject Water transport es_ES
dc.title Study of the Effect of Inorganic Particles on the Gas Transport Properties of Glassy Polyimides for Selective CO2 and H2O Separation es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.3390/membranes8040128 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//SVP-2014-068356/ES/SVP-2014-068356/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//IJCI-2016-28330/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//ENE2014-57651-R/ES/ALMACENAMIENTO DE ENERGIA VIA REDUCCION DE CO2 A COMBUSTIBLES Y PRODUCTOS QUIMICOS/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//SEV-2016-0683/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/GVA//PROMETEO%2F2018%2F006/ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química es_ES
dc.description.bibliographicCitation Escorihuela-Roca, S.; Valero, L.; Tena, A.; Shishatskiy, S.; Escolástico Rozalén, S.; Brinkmann, T.; Serra Alfaro, JM. (2018). Study of the Effect of Inorganic Particles on the Gas Transport Properties of Glassy Polyimides for Selective CO2 and H2O Separation. Membranes. 8(4). https://doi.org/10.3390/membranes8040128 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.3390/membranes8040128 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 8 es_ES
dc.description.issue 4 es_ES
dc.identifier.eissn 2077-0375 es_ES
dc.identifier.pmcid PMC6316831 es_ES
dc.relation.pasarela S\383220 es_ES
dc.contributor.funder Generalitat Valenciana es_ES
dc.contributor.funder Ministerio de Economía y Competitividad es_ES
dc.contributor.funder Helmholtz Association of German Research Centers es_ES
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