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Low-Power Upconversion in Poly(Mannitol-Sebacate) Networks with Tethered Diphenylanthracene and Palladium Porphyrin

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Low-Power Upconversion in Poly(Mannitol-Sebacate) Networks with Tethered Diphenylanthracene and Palladium Porphyrin

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dc.contributor.author Lee, Soo-Hyon es_ES
dc.contributor.author Sonseca, Agueda es_ES
dc.contributor.author Vadrucci, Roberto es_ES
dc.contributor.author Giménez Torres, Enrique es_ES
dc.contributor.author Foster, E.J. es_ES
dc.contributor.author Simon, Yohan C. es_ES
dc.date.accessioned 2020-09-18T03:36:08Z
dc.date.available 2020-09-18T03:36:08Z
dc.date.issued 2014-09 es_ES
dc.identifier.issn 1053-0495 es_ES
dc.identifier.uri http://hdl.handle.net/10251/150354
dc.description.abstract [EN] Efforts to fabricate low-power up converting solid-state systems have rapidly increased in the past decade because of their possible application in several fields such as bio-imaging, drug delivery, solar harvesting or displays. The synthesis of upconverting cross-linked polyester rubbers with covalently tethered chromophores is presented here. Cross-linked films were prepared by reacting a poly(mannitol- sebacate) pre-polymer with 9,10-bis(4-hydroxymethylphenyl) anthracene (DPA-(CH2OH)2) and palladium mesoporphyrin IX. These chromophores served as emitters and sensitizers, respectively, and through a cascade of photophysical events, resulted in an anti-Stokes shifted emission. Indeed, blue emission (*440 nm) of these solid materials was detected upon excitation at 543 nm with a green laser and the power dependence of integrated unconverted intensity versus excitation was examined. The new materials display upconversion at power densities as low as 32 mW/cm2, and do not display phase de-mixing, which has been identified as an obstacle in rubbery blends comprising untethered chromophores. es_ES
dc.description.sponsorship The authors are thankful for the financial support of the Swiss National Science Foundation (200021_13540/1 and 200020_152968), Spanish Ministry of Economy and Competitiveness (Project MAT2010/21494-C03) and the Adolphe Merkle Foundation. The authors thank Prof. Christoph Weder for his help and support. es_ES
dc.language Inglés es_ES
dc.publisher Springer-Verlag es_ES
dc.relation.ispartof Journal of Inorganic and Organometallic Polymers es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject Light upconversion es_ES
dc.subject Triplet triplet annihilation es_ES
dc.subject Poly(mannitol-sebacate)s es_ES
dc.subject Polycondensation es_ES
dc.subject Upconverting elastomer es_ES
dc.subject.classification CIENCIA DE LOS MATERIALES E INGENIERIA METALURGICA es_ES
dc.title Low-Power Upconversion in Poly(Mannitol-Sebacate) Networks with Tethered Diphenylanthracene and Palladium Porphyrin es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1007/s10904-014-0063-7 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/SNSF//200020_152968/CH/Stimuli-Responsive Metal-Containing Polymers/
dc.relation.projectID info:eu-repo/grantAgreement/MICINN//MAT2010-21494-C03-01/ES/DESARROLLO DE ESPUMAS Y SISTEMAS RIGIDOS CON MEMORIA DE FORMA BASADOS EN NANOCOMPUESTOS BIODEGRADABLES NANONOESTRUCTURADOS/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/SNSF//200021_13540%2F1/
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Ingeniería Mecánica y de Materiales - Departament d'Enginyeria Mecànica i de Materials es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto de Tecnología de Materiales - Institut de Tecnologia de Materials es_ES
dc.description.bibliographicCitation Lee, S.; Sonseca, A.; Vadrucci, R.; Giménez Torres, E.; Foster, E.; Simon, YC. (2014). Low-Power Upconversion in Poly(Mannitol-Sebacate) Networks with Tethered Diphenylanthracene and Palladium Porphyrin. Journal of Inorganic and Organometallic Polymers. 24(5):898-903. https://doi.org/10.1007/s10904-014-0063-7 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1007/s10904-014-0063-7 es_ES
dc.description.upvformatpinicio 898 es_ES
dc.description.upvformatpfin 903 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 24 es_ES
dc.description.issue 5 es_ES
dc.relation.pasarela S\283008 es_ES
dc.contributor.funder Adolphe Merkle Foundation es_ES
dc.contributor.funder Swiss National Science Foundation es_ES
dc.contributor.funder Ministerio de Ciencia e Innovación es_ES
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