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Selective catalytic reduction of nitric oxide with ammonia over Fe-Cu modified highly silicated zeolites

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Selective catalytic reduction of nitric oxide with ammonia over Fe-Cu modified highly silicated zeolites

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dc.contributor.author Jouini, Houini es_ES
dc.contributor.author Mejri, Imène es_ES
dc.contributor.author Martinez-Ortigosa, Joaquin es_ES
dc.contributor.author Cerrillo, José Luis es_ES
dc.contributor.author Mhamdi, Mourad es_ES
dc.contributor.author Palomares Gimeno, Antonio Eduardo es_ES
dc.contributor.author Delahay, Gerard es_ES
dc.contributor.author Blasco Lanzuela, Teresa es_ES
dc.date.accessioned 2020-11-11T04:32:10Z
dc.date.available 2020-11-11T04:32:10Z
dc.date.issued 2018-10 es_ES
dc.identifier.issn 1293-2558 es_ES
dc.identifier.uri http://hdl.handle.net/10251/154800
dc.description.abstract [EN] In the present study, the solid-state ion exchange method (SSIE) was applied to introduce iron and copper into highly silicate zeolites: beta (BEA, Si/Al¿=¿12.5), ferrierite (FER, Si/Al¿=¿10) and mordenite (MOR, Si/Al¿=¿10). The activity of the prepared samples in the selective catalytic reduction of NO with ammonia (NH3-SCR) was measured. The highest performance was recorded for Cu-Fe-BEA followed by Cu-Fe-MOR while Cu-Fe-FER showed a low catalytic activity over the entire reaction temperature range. It is shown in this study that the zeolite framework is one of the parameters controlling the amount, environment and distribution of metal species formed during the ion exchange process in Cu-Fe-zeolite catalysts. es_ES
dc.description.sponsorship Financial support by the MINECO of Spain through the Severo Ochoa (SEV-2016-0683) and CTQ2015-68951C3-1-R projects is gratefully acknowledged. The authors thank the Electron Microscopy Service of the Universitat Politecnica de Valencia, Spain for STEM experiments. J. Martinez-Ortigosa (SEV-2012-0267-02) is grateful to Severo Ochoa Program for a predoctoral fellowship. es_ES
dc.language Inglés es_ES
dc.publisher Elsevier es_ES
dc.relation.ispartof Solid State Sciences es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject Si-rich zeolite es_ES
dc.subject Iron es_ES
dc.subject Copper es_ES
dc.subject NH3-SCR es_ES
dc.subject NO es_ES
dc.subject.classification INGENIERIA QUIMICA es_ES
dc.title Selective catalytic reduction of nitric oxide with ammonia over Fe-Cu modified highly silicated zeolites es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1016/j.solidstatesciences.2018.08.008 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//CTQ2015-68951-C3-1-R/ES/TRATAMIENTOS CATALITICOS AVANZADOS PARA LA VALORIZACION DE LA BIOMASA Y LA ELIMINACION DE RESIDUOS ASOCIADOS/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//SEV-2016-0683/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//SEV-2012-0267-02/ es_ES
dc.rights.accessRights Cerrado es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Ingeniería Química y Nuclear - Departament d'Enginyeria Química i Nuclear es_ES
dc.description.bibliographicCitation Jouini, H.; Mejri, I.; Martinez-Ortigosa, J.; Cerrillo, JL.; Mhamdi, M.; Palomares Gimeno, AE.; Delahay, G.... (2018). Selective catalytic reduction of nitric oxide with ammonia over Fe-Cu modified highly silicated zeolites. Solid State Sciences. 84:75-85. https://doi.org/10.1016/j.solidstatesciences.2018.08.008 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1016/j.solidstatesciences.2018.08.008 es_ES
dc.description.upvformatpinicio 75 es_ES
dc.description.upvformatpfin 85 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 84 es_ES
dc.relation.pasarela S\369884 es_ES
dc.contributor.funder Ministerio de Economía y Competitividad es_ES


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