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A Robust Titanium Isophthalate Metal-Organic Framework for Visible-Light Photocatalytic CO2 Methanation

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A Robust Titanium Isophthalate Metal-Organic Framework for Visible-Light Photocatalytic CO2 Methanation

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dc.contributor.author Wang, Sujing es_ES
dc.contributor.author Cabrero-Antonino, Maria es_ES
dc.contributor.author Navalón Oltra, Sergio es_ES
dc.contributor.author Cao, Chen-chen es_ES
dc.contributor.author Tissot, Antoine es_ES
dc.contributor.author Dovgaliuk, Iurii es_ES
dc.contributor.author Marrot, Jerome es_ES
dc.contributor.author Martineau-Corcos, Charlotte es_ES
dc.contributor.author Yu, Liang es_ES
dc.contributor.author Wang, Hao es_ES
dc.contributor.author Shepard, William es_ES
dc.contributor.author García Gómez, Hermenegildo es_ES
dc.contributor.author Serre, Christian es_ES
dc.date.accessioned 2021-05-20T03:33:22Z
dc.date.available 2021-05-20T03:33:22Z
dc.date.issued 2020-12-03 es_ES
dc.identifier.uri http://hdl.handle.net/10251/166524
dc.description.abstract [EN] Isophthalic acid (IPA) has been considered to build metal-organic frameworks (MOFs), owing to its facile availability, unique connection angle-mode, and a wide range of functional groups attached. Constructing titanium-IPA frameworks that possess photoresponse properties is an alluring characteristic with respect to the challenge of synthesizing new titanium-based MOFs (Ti-MOFs) Here, we report the first Ti-IPA MOF (MIP-208) that efficiently combines the use of preformed Ti-8 oxoclusters and in situ acetylation of the 5-NH2-IPA linker. The mixed solid-solution linkers strategy was successfully applied, resulting in a series of multivariate MIP-208 structures with tunable chemical environments and sizable porosity. MIP-208 shows the best result among the pure MOF catalysts for the photocatalytic methanation of carbon dioxide. To improve the photocatalytic performance, ruthenium oxide nanoparticles were photo-deposited on MIP-208, forming a highly active and selective composite catalyst, MIP-208@RuOx, which features a notable visible-light response coupled with excellent stability and recycling ability. es_ES
dc.description.sponsorship S.W. acknowledges the support from the National Natural Science Foundation of China (22071234) and the Fundamental Research Funds for the Central Universities (WK2480000007). S.N. thanks the Ministerio de Ciencia, Innovacion y Universidades (RTI2018-099482-A-I00 project, the Fundacion Ramon Areces (XVIII Concurso Nacional para la Adjudicacion de Ayudas a la Investigacion en Ciencias de la Vida y de la Materia, 2016), and Generalitat Valenciana grupos de investigacion consolidables (AICO/2019/214 project) and Agencia Valenciana de la Innovacion (INNEST/2020/111 project) for financial support. C.-C.C. acknowledges the support from the Program of China Scholarship Council (201700260093) and PHC Cai YuanPei Project (38893VJ). C.M.-C. is grateful for financial support from the Institut Universitaire de France (IUF) and the Paris Ile-de-France Region -DIM "Respore.'' H.G. thanks the Spanish Ministry of Science and Innovation (Severo Ochoa and RTI2018-098237-CO2-1) and Generalitat Valenciana (Prometeo2017/083) for financial support. The authors thank the staff at Synchrotron SOLEIL and the associated scientists for beamtime and assistance during SCXRD data collections on PROXIMA 2A, as well as Dr. Peng Guo and Dr. Nana Yan from Dalian Institute of Chemical Physics (Chinese Academy of Sciences) for the collection of high-resolution PXRD data for Rietveld refinement. es_ES
dc.language Inglés es_ES
dc.publisher Elsevier (Cell Press) es_ES
dc.relation.ispartof Chem es_ES
dc.rights Reconocimiento - No comercial - Sin obra derivada (by-nc-nd) es_ES
dc.subject.classification QUIMICA ORGANICA es_ES
dc.title A Robust Titanium Isophthalate Metal-Organic Framework for Visible-Light Photocatalytic CO2 Methanation es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1016/j.chempr.2020.10.017 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/NSFC//22071234/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/Fundamental Research Funds for the Central Universities//WK2480000007/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/CSC//201700260093/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/Ministère de l'Europe et des Affaires Étrangères//38893VJ/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/GVA//PROMETEO%2F2017%2F083/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/RTI2018-098237-B-C21/ES/HETEROUNIONES DE GRAFENO CON CONFIGURACION CONTROLADA. SINTESIS Y APLICACIONES COMO SOPORTE EN CATALISIS Y EN ELECTRODOS/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/RTI2018-099482-A-I00/ES/DESCOMPOSICION FOTOCATALITICA DEL AGUA ASISTIDA POR LUZ VISIBLE EMPLEANDO MATERIALES NOVEDOSOS Y MULTIFUNCIONALES UIO-66%2F67/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/GVA//AICO%2F2019%2F214/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/AVI//INNEST%2F2020%2F111/ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Química - Departament de Química es_ES
dc.description.bibliographicCitation Wang, S.; Cabrero-Antonino, M.; Navalón Oltra, S.; Cao, C.; Tissot, A.; Dovgaliuk, I.; Marrot, J.... (2020). A Robust Titanium Isophthalate Metal-Organic Framework for Visible-Light Photocatalytic CO2 Methanation. Chem. 6(12):3409-3427. https://doi.org/10.1016/j.chempr.2020.10.017 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1016/j.chempr.2020.10.017 es_ES
dc.description.upvformatpinicio 3409 es_ES
dc.description.upvformatpfin 3427 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 6 es_ES
dc.description.issue 12 es_ES
dc.identifier.eissn 2451-9294 es_ES
dc.relation.pasarela S\430052 es_ES
dc.contributor.funder Region Ile-de-France es_ES
dc.contributor.funder Fundación Ramón Areces es_ES
dc.contributor.funder Generalitat Valenciana es_ES
dc.contributor.funder China Scholarship Council es_ES
dc.contributor.funder Agencia Estatal de Investigación es_ES
dc.contributor.funder Institut Universitaire de France es_ES
dc.contributor.funder Agència Valenciana de la Innovació es_ES
dc.contributor.funder National Natural Science Foundation of China es_ES
dc.contributor.funder Fundamental Research Funds for the Central Universities es_ES
dc.contributor.funder Ministère de l'Europe et des Affaires Étrangères, Francia es_ES
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