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A Pyridyltriazol Functionalized Zirconium Metal-Organic Framework for Selective and Highly Efficient Adsorption of Palladium

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A Pyridyltriazol Functionalized Zirconium Metal-Organic Framework for Selective and Highly Efficient Adsorption of Palladium

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dc.contributor.author Daliran, Saba es_ES
dc.contributor.author Ghazagh-Miri, Mahbobeh es_ES
dc.contributor.author Oveisi, Ali Reza es_ES
dc.contributor.author Khajeh, Mostafa es_ES
dc.contributor.author Navalón Oltra, Sergio es_ES
dc.contributor.author Alvaro Rodríguez, Maria Mercedes es_ES
dc.contributor.author Ghaffari-Moghaddam, Mansour es_ES
dc.contributor.author Delarami, Hojat Samareh es_ES
dc.contributor.author García Gómez, Hermenegildo es_ES
dc.date.accessioned 2021-05-20T03:34:29Z
dc.date.available 2021-05-20T03:34:29Z
dc.date.issued 2020-06-03 es_ES
dc.identifier.issn 1944-8244 es_ES
dc.identifier.uri http://hdl.handle.net/10251/166537
dc.description.abstract [EN] This work reports the synthesis of pyridyltriazol-functionalized UiO-66 (UiO stands for University of Oslo), namely, UiO-66-Pyta, from UiO-66-NH2 through three postsynthetic modification (PSM) steps. The good performance of the material derives from the observation that partial formylation (similar to 21% of -NHCHO groups) of H2BDC-NH2 by DMF, as persistent impurity, takes place during the synthesis of the UiO-66-NH2. Thus, to enhance material performance, first, the as-synthesized UiO-66-NH2 was deformylated to give pure UiO-66-NH2. Subsequently, the pure UiO-66-NH2 was converted to UiO-66-N-3 with a nearly complete conversion (similar to 95%). Finally, the azide-alkyne[3+2]-cycloaddition reaction of 2-ethynylpyridine with the UiO-66-N-3 gave the UiO-66-Pyta. The porous MOF was then applied for the solid-phase extraction of palladium ions from an aqueous medium. Affecting parameters on extraction efficiency of Pd(II) ions were also investigated and optimized. Interestingly, UiO-66-Pyta exhibited selective and superior adsorption capacity for Pd(II) with a maximum sorption capacity of 294.1 mg.g(-1) at acidic pH (4.5). The limit of detection (LOD) was found to be 1.9 mu g L-1. The estimated intra- and interday precisions are 3.6 and 1.7%, respectively. Moreover, the adsorbent was regenerated and reused for five cycles without any significant change in the capacity and repeatability. The adsorption mechanism was described based on various techniques such as FT-IR, PXRD, SEM/EDS, ICP-AES, and XPS analyses as well as density functional theory (DFT) calculations. Notably, as a case study, the obtained UiO-66-Pyta after palladium adsorption, UiO-66-Pyta-Pd, was used as an efficient catalyst for the Suzuki-Miyaura cross-coupling reaction. es_ES
dc.description.sponsorship Authors gratefully acknowledge the financial support for this work from the Politecnica de Valencia, Valencia, Spain. Also, financial support by the University of Zabol is gratefully acknowledged (grant nos. UOZ-GR-9517-1 and UOZ-GR-9618-53). es_ES
dc.language Inglés es_ES
dc.publisher American Chemical Society es_ES
dc.relation.ispartof ACS Applied Materials & Interfaces es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject Zirconium metal-organic framework es_ES
dc.subject UiO-66-NH2 es_ES
dc.subject Pyta-functionalized Zr-MOF es_ES
dc.subject Heavy metal adsorption es_ES
dc.subject Extraction es_ES
dc.subject Density functional theory es_ES
dc.subject Postsynthetic modification es_ES
dc.subject Heterogeneous catalysis es_ES
dc.subject Palladium es_ES
dc.subject.classification QUIMICA ORGANICA es_ES
dc.title A Pyridyltriazol Functionalized Zirconium Metal-Organic Framework for Selective and Highly Efficient Adsorption of Palladium es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1021/acsami.0c06672 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/UOZ//UOZ-GR-9517-1/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/UOZ//UOZ-GR-9618-53/ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Química - Departament de Química es_ES
dc.description.bibliographicCitation Daliran, S.; Ghazagh-Miri, M.; Oveisi, AR.; Khajeh, M.; Navalón Oltra, S.; Alvaro Rodríguez, MM.; Ghaffari-Moghaddam, M.... (2020). A Pyridyltriazol Functionalized Zirconium Metal-Organic Framework for Selective and Highly Efficient Adsorption of Palladium. ACS Applied Materials & Interfaces. 12(22):25221-25232. https://doi.org/10.1021/acsami.0c06672 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1021/acsami.0c06672 es_ES
dc.description.upvformatpinicio 25221 es_ES
dc.description.upvformatpfin 25232 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 12 es_ES
dc.description.issue 22 es_ES
dc.identifier.pmid 32368890 es_ES
dc.relation.pasarela S\430202 es_ES
dc.contributor.funder University of Zabol es_ES
dc.contributor.funder Universitat Politècnica de València es_ES
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