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Influence of Ti Incorporation to Bimetallic Mesoporous Carbon in the Production of 2,5-Dimethylfuran from Biomass Derivatives

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Influence of Ti Incorporation to Bimetallic Mesoporous Carbon in the Production of 2,5-Dimethylfuran from Biomass Derivatives

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dc.contributor.author Ledesma, Brenda C. es_ES
dc.contributor.author Juárez, Juliana M. es_ES
dc.contributor.author Domine, Marcelo Eduardo es_ES
dc.contributor.author Beltramone, Andrea R. es_ES
dc.date.accessioned 2022-12-22T19:00:25Z
dc.date.available 2022-12-22T19:00:25Z
dc.date.issued 2022-05 es_ES
dc.identifier.issn 1011-372X es_ES
dc.identifier.uri http://hdl.handle.net/10251/190903
dc.description.abstract [EN] Monometallic and bimetallic supported catalysts were developed to produce 2,5-dimethylfuran (DMF) trough hydrogenolysis of 5-(hydroxymethyl)furfural (HMF). Detailed physicochemical characterization was done to understand structure-activity correlation. Through a series of experiments and comparatives tests, the synergistic effect among Pt, Ir, and Ti incorporated in the support was investigated. Results revealed that using the titanium contained ordered mesoporous carbon, synthesized by a novel technique, high selectivity to DMF was achieved. In the case of the best catalyst PtIr-TiC, the good activity and excellent selectivity to the desired product DMF (98% yield) was related to the high hydrogenating capacity of the bimetallic sites, the acid support characteristics and the high metal nanoparticles dispersion achieved on the mesoporous titanium modified carbon support. es_ES
dc.description.sponsorship NANOTEC, CONICET, Universidad Tecnologica Nacional, Maestro Lopez y Cruz Roja Argentina. We acknowledge the financial support provided by CONICET Argentina, PIP CONICET 11220120100218CO 2020. M.E.D thanks Spanish Government financial support (CTQ2015-67592 and PGC2018-097277-B-I00). es_ES
dc.language Inglés es_ES
dc.publisher Springer-Verlag es_ES
dc.relation.ispartof Catalysis Letters es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject Titanium es_ES
dc.subject Platinum es_ES
dc.subject Iridium es_ES
dc.subject Modified mesoporous carbon es_ES
dc.subject 5-hydroximethylfurfural es_ES
dc.subject 2,5-dimethylfuran es_ES
dc.title Influence of Ti Incorporation to Bimetallic Mesoporous Carbon in the Production of 2,5-Dimethylfuran from Biomass Derivatives es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1007/s10562-021-03711-8 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PGC2018-097277-B-I00/ES/MEJORA DEL CONCEPTO DE BIORREFINERIA MEDIANTE IMPLEMENTACION DE NUEVOS PROCESOS CATALITICOS CON CATALIZADORES SOLIDOS DE METALES NO NOBLES PARA LA PRODUCCION DE BIOCOMPUESTOS/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/CONICET//11220120100218CO 2020/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//CTQ2015-67592-P/ES/VALORIZACION DE COMPUESTO OXIGENADOS PRESENTES EN FRACCIONES ACUOSAS DERIVADAS DE BIOMASA EN COMBUSTIBLES Y PRODUCTOS QUIMICOS/ es_ES
dc.rights.accessRights Cerrado es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química es_ES
dc.description.bibliographicCitation Ledesma, BC.; Juárez, JM.; Domine, ME.; Beltramone, AR. (2022). Influence of Ti Incorporation to Bimetallic Mesoporous Carbon in the Production of 2,5-Dimethylfuran from Biomass Derivatives. Catalysis Letters. 152(5):1530-1544. https://doi.org/10.1007/s10562-021-03711-8 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1007/s10562-021-03711-8 es_ES
dc.description.upvformatpinicio 1530 es_ES
dc.description.upvformatpfin 1544 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 152 es_ES
dc.description.issue 5 es_ES
dc.relation.pasarela S\463896 es_ES
dc.contributor.funder AGENCIA ESTATAL DE INVESTIGACION es_ES
dc.contributor.funder MINISTERIO DE ECONOMIA Y EMPRESA es_ES
dc.contributor.funder Consejo Nacional de Investigaciones Científicas y Técnicas, Argentina es_ES
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