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Magnetically Induced Catalytic Reduction of Biomass-Derived Oxygenated Compounds in Water

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Magnetically Induced Catalytic Reduction of Biomass-Derived Oxygenated Compounds in Water

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dc.contributor.author Cerezo-Navarrete, Christian es_ES
dc.contributor.author Mustieles Marin, Irene es_ES
dc.contributor.author García-Miquel, Héctor es_ES
dc.contributor.author Corma Canós, Avelino es_ES
dc.contributor.author Chaudret, Bruno es_ES
dc.contributor.author Martínez-Prieto, Luis Miguel es_ES
dc.date.accessioned 2023-05-22T18:02:38Z
dc.date.available 2023-05-22T18:02:38Z
dc.date.issued 2022-07-15 es_ES
dc.identifier.issn 2155-5435 es_ES
dc.identifier.uri http://hdl.handle.net/10251/193517
dc.description.abstract [EN] The development of energetically efficient processes for the aqueous reduction of biomass-derived compounds into chemicals is key for the optimal transformation of biomass. Herein we report an early example of the reduction of biomass-derived oxygenated compounds in water by magnetically induced catalysis. Non-coated and carbon-coated core-shell FeCo@Ni magnetic nanoparticles were used as the heating agent and the catalyst simultaneously. In this way it was possible to control the product distribution by adjusting the field amplitude applied during the magnetic catalysis, opening a precedent for this type of catalysis. Finally, the encapsulation of the magnetic nanoparticles in carbon (FeCo@Ni@C) strongly improved the stability of the magnetic catalyst in solution, making its reuse possible up to at least eight times in dioxane and four times in water. es_ES
dc.description.sponsorship The authors thank the Agencia Estatal de Investigacion (AEI), the Ministerio de Ciencia e Innovacion (MCIN), and the "Ramon y Cajal" program (RYC2020-030031-I) for financial support. The authors also acknowledge an ERC Advanced Grant (MONACAT 2015-694159). C.C.-N. gratefully thanks Generalitat Valenciana for a predoctoral fellowship (GVA: ACIF/2019/076). es_ES
dc.language Inglés es_ES
dc.publisher American Chemical Society es_ES
dc.relation.ispartof ACS Catalysis es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject Magnetic nanoparticles es_ES
dc.subject Core-shell nanoparticles es_ES
dc.subject Magnetically induced catalysis es_ES
dc.subject Hydrogenation reactions es_ES
dc.subject Biomass-derived compounds es_ES
dc.subject.classification TECNOLOGIA ELECTRONICA es_ES
dc.title Magnetically Induced Catalytic Reduction of Biomass-Derived Oxygenated Compounds in Water es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1021/acscatal.2c01696 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/ERC//MONACAT 2015-694159/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/GVA//ACIF%2F2019%2F076/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MICINN//RYC2020-030031-I/ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Escuela Técnica Superior de Ingenieros de Telecomunicación - Escola Tècnica Superior d'Enginyers de Telecomunicació es_ES
dc.description.bibliographicCitation Cerezo-Navarrete, C.; Mustieles Marin, I.; García-Miquel, H.; Corma Canós, A.; Chaudret, B.; Martínez-Prieto, LM. (2022). Magnetically Induced Catalytic Reduction of Biomass-Derived Oxygenated Compounds in Water. ACS Catalysis. 12(14):8462-8475. https://doi.org/10.1021/acscatal.2c01696 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1021/acscatal.2c01696 es_ES
dc.description.upvformatpinicio 8462 es_ES
dc.description.upvformatpfin 8475 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 12 es_ES
dc.description.issue 14 es_ES
dc.relation.pasarela S\475879 es_ES
dc.contributor.funder Generalitat Valenciana es_ES
dc.contributor.funder European Research Council es_ES
dc.contributor.funder Ministerio de Ciencia e Innovación es_ES


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