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Efficient reduction of bromates using carbon nanofibre supported catalysts: experimental and a comparative life cycle assessment study

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Efficient reduction of bromates using carbon nanofibre supported catalysts: experimental and a comparative life cycle assessment study

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dc.contributor.author Yaseneva, Polina es_ES
dc.contributor.author Franch Martí, Cristina es_ES
dc.contributor.author Palomares Gimeno, Antonio Eduardo es_ES
dc.contributor.author Fan, Xiaolei es_ES
dc.contributor.author Morgan, Tobias es_ES
dc.contributor.author Perez, Pablo Saz es_ES
dc.contributor.author Ronning, Magnus es_ES
dc.contributor.author Huang, Fan es_ES
dc.contributor.author Yuranova, Tatiana es_ES
dc.contributor.author Kiwi-Minsker, Liubov es_ES
dc.contributor.author Derrouiche, Salim es_ES
dc.contributor.author Lapkin, Alexei A. es_ES
dc.date.accessioned 2015-09-14T09:30:03Z
dc.date.available 2015-09-14T09:30:03Z
dc.date.issued 2014-07-15
dc.identifier.issn 1385-8947
dc.identifier.uri http://hdl.handle.net/10251/54580
dc.description.abstract [EN] Structured hierarchical catalysts were developed for efficient reduction of bromates in water. In the catalysts a small amount of active metal, 0.3 wt.% Pd, is supported onto carbon nanofibres grown either on sintered metal fibres or on a carbon cloth. In both cases high rates of reaction and high selectivity were achieved, allowing a significant reduction in the amount of catalyst required for the treatment of a set volumetric flow of polluted water, compared to a conventional Pd/Al2O3 catalyst. Manufacture of carbon nanofibres grown on a hierarchical structured support was scaled to 10 g batches. Cradle-to-gate life cycle assessment (LCA) study was performed to compare potential water treatment processes based on two catalyst types, and to identify the areas for future optimisation of the novel technology based on structured hierarchical catalysts. es_ES
dc.description.sponsorship The research leading to these results has received funding from the European Community's Seventh Framework Programme [FP7/2007-2013] for MONACAT under Grant agreement no NMP4-SL-2009-226347. We would like to thank Drs Dana Kralisch and Denise Ott for their advice on Umberto LCA methods.
dc.language Inglés es_ES
dc.publisher Elsevier es_ES
dc.relation.ispartof Chemical Engineering Journal es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject Catalytic reduction of bromates es_ES
dc.subject Water purification es_ES
dc.subject Carbon nanofibres es_ES
dc.subject Nanomaterials es_ES
dc.subject Structured catalysts es_ES
dc.subject Life cycle assessment es_ES
dc.subject.classification INGENIERIA QUIMICA es_ES
dc.title Efficient reduction of bromates using carbon nanofibre supported catalysts: experimental and a comparative life cycle assessment study es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1016/j.cej.2014.03.034
dc.relation.projectID info:eu-repo/grantAgreement/EC/FP7/226347/EU
dc.rights.accessRights Cerrado es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Ingeniería Química y Nuclear - Departament d'Enginyeria Química i Nuclear es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química es_ES
dc.description.bibliographicCitation Yaseneva, P.; Franch Martí, C.; Palomares Gimeno, AE.; Fan, X.; Morgan, T.; Perez, PS.; Ronning, M.... (2014). Efficient reduction of bromates using carbon nanofibre supported catalysts: experimental and a comparative life cycle assessment study. Chemical Engineering Journal. 248:230-241. doi:10.1016/j.cej.2014.03.034 es_ES
dc.description.accrualMethod Senia es_ES
dc.relation.publisherversion http://dx.doi.org/10.1016/j.cej.2014.03.034 es_ES
dc.description.upvformatpinicio 230 es_ES
dc.description.upvformatpfin 241 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 248 es_ES
dc.relation.senia 281954 es_ES
dc.identifier.eissn 1873-3212
dc.contributor.funder European Commission


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