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Constructing Hierarchical Porous Zeolites via Kinetic Regulation

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Constructing Hierarchical Porous Zeolites via Kinetic Regulation

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dc.contributor.author Ding, Kunlun es_ES
dc.contributor.author Corma Canós, Avelino es_ES
dc.contributor.author Maciá Agulló, Juan Antonio es_ES
dc.contributor.author Hu, Jerry G. es_ES
dc.contributor.author Kraemer, Stephan es_ES
dc.contributor.author Stair, Peter C. es_ES
dc.contributor.author Stucky, Galen D. es_ES
dc.date.accessioned 2016-05-10T11:50:39Z
dc.date.issued 2015-09-09
dc.identifier.issn 0002-7863
dc.identifier.uri http://hdl.handle.net/10251/63860
dc.description.abstract Zeolites are crystalline inorganic solids with microporous structures, having widespread applications in the fields of catalysis, separation, adsorption, microelectronics, and medical diagnosis. A major drawback of zeolites is the mass transfer limitation due to the small size of the micropores (less than 1 nm). Numerous efforts have been dedicated to integrating mesopores with the microporous zeolite structures by using templating and/or destructive approaches. Here we provide a new strategy for hierarchical pore size zeolite synthesis, without using supramolecular or hard templates. The branching epitaxial growth behavior, as a result of aluminum-zoning, contributes to the formation of the hierarchical porous zeolite structures. es_ES
dc.description.sponsorship This research was supported by the University of California Discovery Grant Program GCP08-128649 (to K.D. and G.D.S.) and the U.S. National Science Foundation CHE-1058835 (to K.D. and P.C.S.). A.C. thanks the program Severo Ochoa for financial support. J.A.M.-A. acknowledges the assistance of the CSIC for the award of a Postdoctoral JAE-Doc contract. This research made extensive usage of the Shared Experimental Facilities of the Materials Research Laboratory, which are supported by the MRSEC Program of the NSF under Award No. DMR 1121053; a member of the NSF-funded Materials Research Facilities Network (www.mrfn.org). en_EN
dc.language Inglés es_ES
dc.publisher American Chemical Society es_ES
dc.relation University of California Discovery Grant Program GCP08-128649 es_ES
dc.relation U.S. National Science Foundation CHE-1058835 es_ES
dc.relation program Severo Ochoa es_ES
dc.relation MRSEC Program of the NSF DMR 1121053 es_ES
dc.relation CSIC es_ES
dc.relation.ispartof Journal of the American Chemical Society es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject HYDROTHERMAL SYNTHESIS es_ES
dc.subject MESOPOROUS CHANNELS es_ES
dc.subject SINGLE-CRYSTALS es_ES
dc.subject ZSM-5 CRYSTALS es_ES
dc.subject ALUMINUM es_ES
dc.subject ARCHITECTURES es_ES
dc.subject NANOSHEETS es_ES
dc.subject.classification QUIMICA ORGANICA es_ES
dc.title Constructing Hierarchical Porous Zeolites via Kinetic Regulation es_ES
dc.type Artículo es_ES
dc.embargo.lift 10000-01-01
dc.embargo.terms forever es_ES
dc.identifier.doi 10.1021/jacs.5b06791
dc.rights.accessRights Cerrado es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Química - Departament de Química es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química es_ES
dc.description.bibliographicCitation Ding, K.; Corma Canós, A.; Maciá Agulló, JA.; Hu, JG.; Kraemer, S.; Stair, PC.; Stucky, GD. (2015). Constructing Hierarchical Porous Zeolites via Kinetic Regulation. Journal of the American Chemical Society. 137(35):11238-11241. doi:10.1021/jacs.5b06791 es_ES
dc.description.accrualMethod Senia es_ES
dc.relation.publisherversion http://dx.doi.org/10.1021/jacs.5b06791 es_ES
dc.description.upvformatpinicio 11238 es_ES
dc.description.upvformatpfin 11241 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 137 es_ES
dc.description.issue 35 es_ES
dc.relation.senia 309291 es_ES


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