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Promoted hexagonal tungsten bronzes as selective catalysts in the aerobic transformation of alcohols: glycerol and methanol

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Promoted hexagonal tungsten bronzes as selective catalysts in the aerobic transformation of alcohols: glycerol and methanol

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dc.contributor.author Soriano Rodríguez, Mª Dolores es_ES
dc.contributor.author Chieregato, A. es_ES
dc.contributor.author Zamora Blanco, Segundo es_ES
dc.contributor.author Basile, F. es_ES
dc.contributor.author Cavani, F. es_ES
dc.contributor.author López Nieto, José Manuel es_ES
dc.date.accessioned 2016-05-17T07:23:05Z
dc.date.available 2016-05-17T07:23:05Z
dc.date.issued 2016-02
dc.identifier.issn 1022-5528
dc.identifier.uri http://hdl.handle.net/10251/64177
dc.description.abstract [EN] M-containing tungsten oxides bronzes (M = Ti, Nb or V) with hexagonal tungsten bronze (HTB) structure have been investigated as catalysts for the aerobic transformation of glycerol and methanol. The catalysts were prepared hydrothermally and characterized by several physico chemical techniques, i.e. N-2-adsorption, XRD, Raman spectroscopy and temperature programmed desorption of ammonia. Interesting variations in the thermal stability of the HTB-framework were observed according to the element introduced into the oxide structure. In addition, the incorporation of Ti and Nb modified the acid features of the hexagonal tungsten oxides, whereas V introduced new redox sites. The catalytic results for the aerobic transformation of glycerol and methanol in terms of conversion and nature of reaction products are discussed on the basis of the physicochemical characteristics of catalysts. es_ES
dc.description.sponsorship JMLN and MDS thank the Spanish Government-MINECO (CTQ2012-37925-C03-1 and program Severo Ochoa SEV-2012-0267). CIRI and INSTM are acknowledged for the grant to AC.
dc.language Inglés es_ES
dc.publisher Springer Verlag (Germany) es_ES
dc.relation.ispartof Topics in Catalysis es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject Vanadium, tiutanium and niobium promoters es_ES
dc.subject Hexagonal tungsten bronzes es_ES
dc.subject Selective catalysts es_ES
dc.subject Aerobic transformation of alcohols: glycerol and methanol es_ES
dc.subject Metal oxides es_ES
dc.subject Bronze es_ES
dc.subject Tungsten es_ES
dc.subject Aerobic transformation es_ES
dc.subject Methanol es_ES
dc.subject Glycerol es_ES
dc.title Promoted hexagonal tungsten bronzes as selective catalysts in the aerobic transformation of alcohols: glycerol and methanol es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1007/s11244-015-0440-7
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//CTQ2012-37925-C03-01/ES/CATALIZADORES PARA LA ENERGIA Y EL MEDIOAMBIENTE: ACTIVACION SELECTIVA DE ENLACES S-H Y C-H/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//SEV-2012-0267/ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química es_ES
dc.description.bibliographicCitation Soriano Rodríguez, MD.; Chieregato, A.; Zamora Blanco, S.; Basile, F.; Cavani, F.; López Nieto, JM. (2016). Promoted hexagonal tungsten bronzes as selective catalysts in the aerobic transformation of alcohols: glycerol and methanol. Topics in Catalysis. 59(2-4):178-185. https://doi.org/10.1007/s11244-015-0440-7 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion http://dx.doi.org/10.1007/s11244-015-0440-7 es_ES
dc.description.upvformatpinicio 178 es_ES
dc.description.upvformatpfin 185 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 59 es_ES
dc.description.issue 2-4 es_ES
dc.relation.senia 302273 es_ES
dc.contributor.funder Ministerio de Economía y Competitividad
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