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Promoted NiO catalysts for the oxidative dehydrogenation of ethane

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Promoted NiO catalysts for the oxidative dehydrogenation of ethane

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dc.contributor.author López Nieto, José Manuel es_ES
dc.contributor.author Solsona Espriu, Benjamin Eduardo es_ES
dc.contributor.author Grasselli, Robert K. es_ES
dc.contributor.author Concepción Heydorn, Patricia es_ES
dc.date.accessioned 2016-05-17T07:29:47Z
dc.date.available 2016-05-17T07:29:47Z
dc.date.issued 2014-09
dc.identifier.issn 1022-5528
dc.identifier.uri http://hdl.handle.net/10251/64186
dc.description.abstract Metal oxide promoted NiO catalysts with a Ni/(Me + Ni) atomic ratio 0.92 have been investigated for the oxidative dehydrogenation of ethane. These materials have been characterized by several techniques (N-2-adsorption, X-ray diffraction, X-ray photoelectron spectroscopy and Fourier transformed infrared spectroscopy of adsorbed CO and ethylene). The nature of surface sites is strongly influenced by the valence and the acid/base characteristics of the metal oxide promoters, which have a great impact on the selectivity to ethylene. Accordingly, a clear correlation between selectivity to ethylene and the valence of the promoter has been observed in the present work. Additionally, the acidity of the catalyst also enhances the selectivity to ethylene. es_ES
dc.description.sponsorship The Spanish authors would like to thank the DGICYT in Spain (Project CTQ2012-37925-C03-1 and CTQ2012-37925-C03-2) for financial support. en_EN
dc.language Inglés es_ES
dc.publisher Springer Verlag (Germany) es_ES
dc.relation.ispartof Topics in Catalysis es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject Promoted NiO catalysts es_ES
dc.subject Nickel oxide es_ES
dc.subject Oxidative dehydrogenation es_ES
dc.subject Ethane es_ES
dc.subject Ethylene es_ES
dc.subject Valence es_ES
dc.subject Promoters es_ES
dc.subject Acidity and basicity es_ES
dc.title Promoted NiO catalysts for the oxidative dehydrogenation of ethane es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1007/s11244-014-0288-2
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//CTQ2012-37925-C03-01/ES/CATALIZADORES PARA LA ENERGIA Y EL MEDIOAMBIENTE: ACTIVACION SELECTIVA DE ENLACES S-H Y C-H/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//CTQ2012-37925-C03-02/ES/CATALIZADORES PARA LA ENERGIA Y EL MEDIOAMBIENTE: OPTIMIZACION DE PROCESOS CATALITICOS DE OXIDACION PARA LA OBTENCION DE HIDROGENO Y OLEFINAS Y LA ELIMINACION DE VOCS./ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química es_ES
dc.description.bibliographicCitation López Nieto, JM.; Solsona Espriu, BE.; Grasselli, RK.; Concepción Heydorn, P. (2014). Promoted NiO catalysts for the oxidative dehydrogenation of ethane. Topics in Catalysis. 57(14-16):1248-1255. https://doi.org/10.1007/s11244-014-0288-2 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion http://dx.doi.org/10.1007/s11244-014-0288-2 es_ES
dc.description.upvformatpinicio 1248 es_ES
dc.description.upvformatpfin 1255 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 57 es_ES
dc.description.issue 14-16 es_ES
dc.relation.senia 289556 es_ES
dc.contributor.funder Ministerio de Economía y Competitividad es_ES
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