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Beyond Acid Strength in Zeolites: Soft Framework Counteranions for Stabilization of Carbocations on Zeolites and Its Implication in Organic Synthesis

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Beyond Acid Strength in Zeolites: Soft Framework Counteranions for Stabilization of Carbocations on Zeolites and Its Implication in Organic Synthesis

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Cabrero Antonino, JR.; Leyva Perez, A.; Corma Canós, A. (2015). Beyond Acid Strength in Zeolites: Soft Framework Counteranions for Stabilization of Carbocations on Zeolites and Its Implication in Organic Synthesis. Angewandte Chemie International Edition. 54(19):5658-5661. doi:10.1002/anie.201500864

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Title: Beyond Acid Strength in Zeolites: Soft Framework Counteranions for Stabilization of Carbocations on Zeolites and Its Implication in Organic Synthesis
Author:
UPV Unit: Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química
Universitat Politècnica de València. Departamento de Química - Departament de Química
Issued date:
Abstract:
[EN] The generation of a carbocation with an acid depends not only on the acid strength but also on the ability of the counteranion to stabilize the positive charge left behind. Here we report that despite their relatively ...[+]
Subjects: Carbocations , Cycloaddition reactions , Heterogeneous catalysis , Propargyl alcohols , zeolites
Copyrigths: Reserva de todos los derechos
Source:
Angewandte Chemie International Edition. (issn: 1433-7851 ) (eissn: 1521-3773 )
DOI: 10.1002/anie.201500864
Publisher:
Wiley
Publisher version: https://dx.doi.org/10.1002/anie.201500864
Thanks:
This work was supported by Consolider-Ingenio 2010 (proyecto MULTICAT) and Severo Ochoa program. J.R.C.-A. and A. L.-P. thank ITQ for a fellowship. We thank Dr. S. Valencia for providing H-Beta nanocrystalline zeolite and ...[+]
Type: Artículo

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