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Surface-Mediated Synthesis of Dimeric Rhodium Catalysts on MgO: Tracking Changes in the Nuclearity and Ligand Environment of the Catalytically Active Sites by X-ray Absorption and Infrared Spectroscopies

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Surface-Mediated Synthesis of Dimeric Rhodium Catalysts on MgO: Tracking Changes in the Nuclearity and Ligand Environment of the Catalytically Active Sites by X-ray Absorption and Infrared Spectroscopies

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Yardimci, D.; Serna Merino, PM.; Gates, BC. (2013). Surface-Mediated Synthesis of Dimeric Rhodium Catalysts on MgO: Tracking Changes in the Nuclearity and Ligand Environment of the Catalytically Active Sites by X-ray Absorption and Infrared Spectroscopies. Chemistry - A European Journal. 19(4):1235-1245. doi:10.1002/chem.201202514

Por favor, use este identificador para citar o enlazar este ítem: http://hdl.handle.net/10251/66415

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Title: Surface-Mediated Synthesis of Dimeric Rhodium Catalysts on MgO: Tracking Changes in the Nuclearity and Ligand Environment of the Catalytically Active Sites by X-ray Absorption and Infrared Spectroscopies
Author:
UPV Unit: Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química
Issued date:
Abstract:
[EN] The preparation of dinuclear rhodium clusters and their use as catalysts is challenging because these clusters are unstable, evolving readily into species with higher nuclearities. We now present a novel synthetic ...[+]
Subjects: Catalysis , Cluster compounds , Dimerization , Hydrogenation , Rhodium , Supported catalysts
Copyrigths: Cerrado
Source:
Chemistry - A European Journal. (issn: 0947-6539 )
DOI: 10.1002/chem.201202514
Publisher:
Wiley
Publisher version: http://dx.doi.org/10.1002/chem.201202514
Project ID: info:eu-repo/grantAgreement/EC/FP7/253129/EU
Thanks:
The research was supported by the European Union Seventh Framework Programme (FP7/2007-2013) under grant agreement no. PIOF-GA-2009-253129 (P. S.) and by DOE Basic Energy Sciences (Contract No. FG02-04ER15513) (D.Y.). We ...[+]
Type: Artículo

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