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Factors Controlling the Acidity of Zeolites

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Factors Controlling the Acidity of Zeolites

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dc.contributor.author Boronat Zaragoza, Mercedes es_ES
dc.contributor.author Corma Canós, Avelino es_ES
dc.date.accessioned 2016-10-17T08:35:50Z
dc.date.available 2016-10-17T08:35:50Z
dc.date.issued 2015-01
dc.identifier.issn 1011-372X
dc.identifier.uri http://hdl.handle.net/10251/71893
dc.description.abstract Most industrial applications of zeolites as catalysts rely on their Bronsted acidity properties. However, neither quantifying acid strength in solids nor correlating acidity with catalytic activity is straightforward. The ease and speed at which the proton transfer process occurs in zeolites depends on different factors, including the concentration of active sites and local geometry around them, the ability of base molecules to diffuse through channels and cavities close to the acid sites, and the stabilization of ionic transition states and intermediates by electrostatic interactions with the zeolite framework. All these aspects are analyzed in this review based on experimental characterization data (FTIR spectroscopy of hydroxyl groups and adsorbed probe molecules, in situ MAS-NMR of reactants and intermediates, TPD and microcalorimetry of adsorbed probe molecules) and computational studies. es_ES
dc.description.sponsorship The authors thank the Spanish Science and Innovation Ministry (Consolider Ingenio 2010-MULTICAT CSD2009-00050 Project and Subprograma de apoyo a Centros y Universidades de Excelencia Severo Ochoa SEV 2012 0267) and Generalitat Valenciana (PROMETEOII/2013/011 Project) for financial support. en_EN
dc.language Inglés es_ES
dc.publisher Springer Verlag es_ES
dc.relation.ispartof Catalysis Letters es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject Catalysis es_ES
dc.subject Zeolites es_ES
dc.subject Bronsted acidity es_ES
dc.subject Reactivity es_ES
dc.subject.classification QUIMICA ORGANICA es_ES
dc.title Factors Controlling the Acidity of Zeolites es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1007/s10562-014-1438-7
dc.relation.projectID info:eu-repo/grantAgreement/MICINN//CSD2009-00050/ES/Desarrollo de catalizadores más eficientes para el diseño de procesos químicos sostenibles y produccion limpia de energia/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/GVA//PROMETEOII%2F2013%2F011/ES/Catalizadores moleculares y supramoleculares altamente selectivos, estables y energéticamente eficientes en reacciones químicas (PROMETEO)/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//SEV-2012-0267/ES/SEV-2012-0267/ es_ES
dc.rights.accessRights Cerrado es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Química - Departament de Química es_ES
dc.description.bibliographicCitation Boronat Zaragoza, M.; Corma Canós, A. (2015). Factors Controlling the Acidity of Zeolites. Catalysis Letters. 145(1):162-172. https://doi.org/10.1007/s10562-014-1438-7 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion http://dx.doi.org/10.1007/s10562-014-1438-7 es_ES
dc.description.upvformatpinicio 162 es_ES
dc.description.upvformatpfin 172 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 145 es_ES
dc.description.issue 1 es_ES
dc.relation.senia 309148 es_ES
dc.identifier.eissn 1572-879X
dc.contributor.funder Generalitat Valenciana es_ES
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