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A Combined Experimental and Theoretical Approach to the Photogeneration of 5,6-Dihydropyrimidin-5-yl Radicals in Nonaqueous Media

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A Combined Experimental and Theoretical Approach to the Photogeneration of 5,6-Dihydropyrimidin-5-yl Radicals in Nonaqueous Media

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Aparici-Espert, MI.; Francés Monerris, A.; Rodríguez Muñiz, GM.; Roca Sanjuan, D.; Lhiaubet, VL.; Miranda Alonso, MÁ. (2016). A Combined Experimental and Theoretical Approach to the Photogeneration of 5,6-Dihydropyrimidin-5-yl Radicals in Nonaqueous Media. Journal of Organic Chemistry. 81(10):4031-4038. doi:10.1021/acs.joc.6b00314

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Title: A Combined Experimental and Theoretical Approach to the Photogeneration of 5,6-Dihydropyrimidin-5-yl Radicals in Nonaqueous Media
Author:
UPV Unit: Universitat Politècnica de València. Escuela Técnica Superior de Ingenieros Industriales - Escola Tècnica Superior d'Enginyers Industrials
Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química
Universitat Politècnica de València. Departamento de Química - Departament de Química
Issued date:
Abstract:
The chemical fate of radical intermediates is relevant to understand the biological effects of radiation and to explain formation of DNA lesions. A direct approach to selectively generate the putative reactive intermediates ...[+]
Subjects: 2ND-ORDER PERTURBATION-THEORY , HYDROGEN-ATOM ABSTRACTION , INDEPENDENT GENERATION , STRAND SCISSION , DNA-DAMAGE , AQUEOUS-SOLUTIONS , RADIATION , REPAIR , THYMIDINE , 5,6-DIHYDROTHYMID-5-YL
Copyrigths: Cerrado
Source:
Journal of Organic Chemistry. (issn: 0022-3263 )
DOI: 10.1021/acs.joc.6b00314
Publisher:
American Chemical Society
Publisher version: http://doi.org/10.1021/acs.joc.6b00314
Thanks:
Spanish Government (CTQ2012-32621, CTQ2015-70164-P, CTQ2014-58624-P, RIRAAF RETICS RD12/0013/0009, Severo Ochoa program/SEV-2012-0267, Maria de Maetzu program/MDM-2015-0538, BES-2011-048326 and BES-2013-066566, JCI-2012-13431) ...[+]
Type: Artículo

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