Production strategies of asymmetric BaCe0.65Zr0.20Y0.15O3-delta - Ce(0.8)Gd(0.2)O(2-delta) membrane for hydrogen separation
| dc.contributor.affiliation | Instituto Universitario Mixto de Tecnología Química | |
| dc.contributor.author | Mercadelli, Elisa | es_ES |
| dc.contributor.author | Gondolini, Angela | es_ES |
| dc.contributor.author | Montaleone, Daniel | es_ES |
| dc.contributor.author | Pinasco, Paola | es_ES |
| dc.contributor.author | Escolástico Rozalén, Sonia | |
| dc.contributor.author | Serra Alfaro, José Manuel | |
| dc.contributor.author | Sanson, Alessandra | es_ES |
| dc.date.accessioned | 2021-02-10T04:31:37Z | |
| dc.date.available | 2021-02-10T04:31:37Z | |
| dc.date.issued | 2020-03-04 | es_ES |
| dc.description.abstract | [EN] Mixed proton and electron conductor ceramic composites are among the most promising materials for hydrogen separation membrane technology especially if designed in an asymmetrical configuration (thin membrane supported onto a thicker porous substrate). However a precise processing optimization is needed to effectively obtain planar and crack free asymmetrical membranes with suitable microstructure and composition without affecting their hydrogen separation efficiency. This work highlights for the first time the most critical issues linked to the tape casting process used to obtain BaCe0.65Zr0.20Y0.15O3-delta - Ce0.8Gd0.2O2-delta (BCZY-GDC) asymmetrical membranes for H-2 separation. The critical role of the co-firing process, sintering aid and atmosphere was critically investigated. The optimization of the production strategy allowed to obtain asymmetric membranes constituted by a dense 20 mu m-thick ceramic-ceramic composite layer supported by a porous (36%) 750 mu m-thick BCZY-GDC substrate. The asymmetric membranes here reported showed H2 fluxes (0.47 mL min(-1) cm(-2) at 750 degrees C) among the highest obtained for an all-ceramic membrane. | en_EN |
| dc.description.accrualMethod | S | es_ES |
| dc.description.bibliographicCitation | Mercadelli, E.; Gondolini, A.; Montaleone, D.; Pinasco, P.; Escolástico Rozalén, S.; Serra Alfaro, JM.; Sanson, A. (2020). Production strategies of asymmetric BaCe0.65Zr0.20Y0.15O3-delta - Ce(0.8)Gd(0.2)O(2-delta) membrane for hydrogen separation. International Journal of Hydrogen Energy. 45(12):7468-7478. https://doi.org/10.1016/j.ijhydene.2019.03.148 | es_ES |
| dc.description.issue | 12 | es_ES |
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| dc.description.sponsorship | This work has been funded by the agreement between the Italian Ministry of Economic Development and the Italian National Research Council "Ricerca di sistema elettrico nazionale" | es_ES |
| dc.description.upvformatpfin | 7478 | es_ES |
| dc.description.upvformatpinicio | 7468 | es_ES |
| dc.description.volume | 45 | es_ES |
| dc.identifier.doi | 10.1016/j.ijhydene.2019.03.148 | es_ES |
| dc.identifier.issn | 0360-3199 | es_ES |
| dc.identifier.uri | https://riunet.upv.es/handle/10251/160984 | |
| dc.language | Inglés | es_ES |
| dc.publisher | Elsevier | es_ES |
| dc.relation.ispartof | International Journal of Hydrogen Energy | es_ES |
| dc.relation.pasarela | S\417947 | es_ES |
| dc.relation.publisherversion | https://doi.org/10.1016/j.ijhydene.2019.03.148 | es_ES |
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| dc.rights | Reconocimiento - No comercial - Sin obra derivada (by-nc-nd) | es_ES |
| dc.rights.accessRights | Abierto | es_ES |
| dc.subject | Tape casting | es_ES |
| dc.subject | BCZY-GDC | es_ES |
| dc.subject | Ceramic membranes | es_ES |
| dc.subject | Microstructure | es_ES |
| dc.title | Production strategies of asymmetric BaCe0.65Zr0.20Y0.15O3-delta - Ce(0.8)Gd(0.2)O(2-delta) membrane for hydrogen separation | es_ES |
| dc.type | Artículo | es_ES |
| dc.type.version | info:eu-repo/semantics/publishedVersion | es_ES |
| dspace.entity.type | Publication | |
| person.identifier | 61212 | |
| person.identifier | 41579 | |
| person.identifier.orcid | 0000-0002-7097-2425 | |
| person.identifier.orcid | 0000-0002-1515-1106 | |
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