High-silica nanocrystalline Beta zeolites: efficient synthesis and catalytic application

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dc.contributor.affiliationInstituto Universitario Mixto de Tecnología Química
dc.contributor.authorMartínez Franco, Raqueles_ES
dc.contributor.authorParis, Cecilia
dc.contributor.authorMartínez Armero, Marta Eveliaes_ES
dc.contributor.authorMartínez, Cristina
dc.contributor.authorMoliner Marin, Manuel
dc.contributor.authorCorma Canós, Avelino
dc.contributor.funderMinisterio de Economía y Competitividades_ES
dc.contributor.funderEuropean Commissiones_ES
dc.date.accessioned2018-03-11T05:03:33Z
dc.date.available2018-03-11T05:03:33Z
dc.date.issued2015es_ES
dc.description.abstract[EN] An efficient synthesis methodology to obtain homogeneous nanosized high-silica Beta zeolites ( 10¿20 nm) with high solid yields (above 95%) using simple alkyl-substituted flexible dicationic OSDAs is described. These dicationic OSDAs allow the synthesis of nanosized Beta zeolites with different Si/Al ratios (15¿30) in alkaline and fluoride media, resulting in nanocrystalline materials with different physicochemical properties. These nanosized Beta zeolites show better catalytic behavior towards the industrially-relevant alkylation of benzene with propylene to obtain cumene compared with other commercially available nanosized Beta zeolites.en_EN
dc.description.accrualMethodSes_ES
dc.description.bibliographicCitationMartínez Franco, R.; Paris-Carrizo, CG.; Martínez Armero, ME.; Martínez, C.; Moliner Marin, M.; Corma Canós, A. (2015). High-silica nanocrystalline Beta zeolites: efficient synthesis and catalytic application. Chemical Science. 7(1):102-108. https://doi.org/10.1039/c5sc03019fes_ES
dc.description.issue1es_ES
dc.description.sponsorshipFinancial support from the Spanish Government-MINECO through “Severo Ochoa” (SEV 2012-0267), Consolider Ingenio 2010-Multicat, MAT2012-37160 and, MAT2012-31657 is acknowledged. The European Union is also acknowledged by the SynCatMatch project (ERC-AdG-2014-671093). M.E.M-A. thanks MINECO for economical support through a pre-doctoral fellowship (BES-2013-066800).
dc.description.upvformatpfin108es_ES
dc.description.upvformatpinicio102es_ES
dc.description.volume7es_ES
dc.identifier.doi10.1039/c5sc03019fes_ES
dc.identifier.issn2041-6520es_ES
dc.identifier.pmcidPMC5950835en_EN
dc.identifier.pmid29861970en_EN
dc.identifier.urihttps://riunet.upv.es/handle/10251/99143
dc.languageIngléses_ES
dc.publisherThe Royal Society of Chemistryes_ES
dc.relation.ispartofChemical Sciencees_ES
dc.relation.pasarelaS\296982es_ES
dc.relation.projectIDinfo:eu-repo/grantAgreement/MINECO//MAT2012-31657/ES/SINTESIS DE ZEOLITAS MEDIANTE AGENTES DIRECTORES DE ESTRUCTURA BASADOS EN ?MIMICOS? DE ESTADOS DE TRANSICION DE REACCIONES DE INTERES INDUSTRIAL/es_ES
dc.relation.projectIDinfo:eu-repo/grantAgreement/EC/H2020/671093/EU/MATching zeolite SYNthesis with CATalytic activity/es_ES
dc.relation.projectIDinfo:eu-repo/grantAgreement/MINECO//MAT2012-37160/ES/SINTESIS DE NUEVOS MATERIALES MICROPOROSOS BASADOS EN EL USO DE ?ESPONJAS DE PROTONES? COMO AGENTES DIRECTORES DE ESTRUCTURA (ADES)/es_ES
dc.relation.projectIDinfo:eu-repo/grantAgreement/MINECO//SEV-2012-0267/es_ES
dc.relation.projectIDinfo:eu-repo/grantAgreement/MINECO//BES-2013-066800/ES/BES-2013-066800/es_ES
dc.relation.publisherversionhttps://doi.org/10.1039/c5sc03019fes_ES
dc.rightsReconocimiento (by)es_ES
dc.rights.accessRightsAbiertoes_ES
dc.subject.classificationQUIMICA ORGANICAes_ES
dc.titleHigh-silica nanocrystalline Beta zeolites: efficient synthesis and catalytic applicationes_ES
dc.typeArtículoes_ES
dc.type.versioninfo:eu-repo/semantics/publishedVersiones_ES
dspace.entity.typePublication
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