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Intracrystalline diffusion in metal organic framework during heterogeneous catalisys: Influence of particle size on the activity of MIL-100 (Fe) for oxidation reaction

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Intracrystalline diffusion in metal organic framework during heterogeneous catalisys: Influence of particle size on the activity of MIL-100 (Fe) for oxidation reaction

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Dhakshinamoorthy, A.; Alvaro Rodríguez, MM.; Hwang, YK.; Seo, Y.; Corma Canós, A.; García Gómez, H. (2011). Intracrystalline diffusion in metal organic framework during heterogeneous catalisys: Influence of particle size on the activity of MIL-100 (Fe) for oxidation reaction. Dalton Transactions. 40(40):10719-10724. https://doi.org/10.1039/c1dt10826c

Por favor, use este identificador para citar o enlazar este ítem: http://hdl.handle.net/10251/105404

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Título: Intracrystalline diffusion in metal organic framework during heterogeneous catalisys: Influence of particle size on the activity of MIL-100 (Fe) for oxidation reaction
Autor: Dhakshinamoorthy, Amarajothi Alvaro Rodríguez, Maria Mercedes Hwang, Young Kyu Seo, You-Kyong Corma Canós, Avelino García Gómez, Hermenegildo
Entidad UPV: Universitat Politècnica de València. Departamento de Química - Departament de Química
Fecha difusión:
Resumen:
[EN] Three MIL-100 (Fe) samples differing in average crystal size (from 60-70 to >400 nm) have been synthesized by microwave heating using three HF/Fe 3+ ratios. Oxidation of diphenylmethane with tert-butylhydroperoxide ...[+]
Palabras clave: Average particle size , Crystal size , Diffusion limitations , Diphenylmethane , Intracrystalline diffusion , Intracrystalline space , Oxidation reactions , Porous catalysts , Substrate sizes , Tert-butylhydroperoxide , Thiophenols , Grain size and shape , Organometallics , Oxidation , Particle size , Reaction rates , Catalysis , benzhydryl derivative , Ferric ion , Metal , Organic compound , Oxygen , Phenol derivative , Tert butyl hydroperoxide , Thiol derivative , Thiophenol , Article , Chemistry , diffusion , oxidation reduction reaction , synthesis , Benzhydryl Compounds , Ferric Compounds , Metals , Organic Chemicals , Oxidation-Reduction , Phenols , Sulfhydryl Compounds
Derechos de uso: Cerrado
Fuente:
Dalton Transactions. (issn: 1477-9226 )
DOI: 10.1039/c1dt10826c
Editorial:
ROYAL SOC CHEMISTRY
Versión del editor: http://doi.org/10.1039/c1dt10826c
Código del Proyecto:
info:eu-repo/grantAgreement/MICINN//CTQ2010-18671/ES/APLICACION DE SOLIDOS RETICULARES METAL-ORGANICO MODIFICADOS COMO CATALIZADORES HETEROGENEOS EN PROCESOS DE OXIDACION AEROBICA Y EN REACCIONES PROMOVIDAS POR ACIDOS DE LEWIS/
Ministerio de Economía, Industria y Competitividad/CTQ2009--11587
Agradecimientos:
Financial support by the Spanish DGI (CTQ2009-11587 and CTQ2010-18671 and Consolider MULTICAT) is gratefully acknowledged. Prof. Jong-San Chang and his group are thanked for providing us with sufficient quantities of the ...[+]
Tipo: Artículo

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