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A heterogeneous mechanism for the catalytic decomposition of hydroperoxides and oxidation of alkanes over CeO2 nanoparticles: A combined theoretical and experimental study

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A heterogeneous mechanism for the catalytic decomposition of hydroperoxides and oxidation of alkanes over CeO2 nanoparticles: A combined theoretical and experimental study

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López Auséns, JT.; Boronat Zaragoza, M.; Concepción Heydorn, P.; Chouzier, S.; Mastroianni, S.; Corma Canós, A. (2016). A heterogeneous mechanism for the catalytic decomposition of hydroperoxides and oxidation of alkanes over CeO2 nanoparticles: A combined theoretical and experimental study. Journal of Catalysis. 344:334-345. doi:10.1016/j.jcat.2016.09.032

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Title: A heterogeneous mechanism for the catalytic decomposition of hydroperoxides and oxidation of alkanes over CeO2 nanoparticles: A combined theoretical and experimental study
Author:
UPV Unit: Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química
Universitat Politècnica de València. Departamento de Química - Departament de Química
Issued date:
Abstract:
[EN] A nanoparticulate CeO2 catalyst is presented that is able to oxidize cyclohexane to K/A-oil (a mixture of cyclohexanone and cyclohexanol) using hydroperoxides as oxidizing species. The improvement in selectivity with ...[+]
Subjects: Alkane oxidation , Heterogeneous catalysis , Acid-base , Redox , Ceria , DFT , in situ IR , Electron Microscopy Service of the UPV
Copyrigths: Cerrado
Source:
Journal of Catalysis. (issn: 0021-9517 )
DOI: 10.1016/j.jcat.2016.09.032
Publisher:
Elsevier
Publisher version: https://doi.org/10.1016/j.jcat.2016.09.032
Project ID: info:eu-repo/grantAgreement/EC/H2020/671093/EU
Thanks:
The authors thank Solvay, MINECO (Consolider Ingenio 2010-MULTICAT, CSD2009-00050 and Severo Ochoa program, SEV-2012-0267), Generalitat Valenciana (PROMETEOII/2013/011 Project) and the European Union (ERC-AdG-2014-671093 ...[+]
Type: Artículo

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