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dc.contributor.author | Delgado, T.![]() |
es_ES |
dc.contributor.author | Meneses-Sánchez, M.![]() |
es_ES |
dc.contributor.author | Piñeiro-López, L.![]() |
es_ES |
dc.contributor.author | Bartual-Murgui, C.![]() |
es_ES |
dc.contributor.author | Muñoz Roca, María Del Carmen![]() |
es_ES |
dc.contributor.author | Real, J.A.![]() |
es_ES |
dc.date.accessioned | 2020-07-08T03:32:39Z | |
dc.date.available | 2020-07-08T03:32:39Z | |
dc.date.issued | 2018-11-28 | es_ES |
dc.identifier.issn | 2041-6520 | es_ES |
dc.identifier.uri | http://hdl.handle.net/10251/147639 | |
dc.description.abstract | [EN] The search for bifunctional materials showing synergies between spin crossover (SCO) and luminescence has attracted substantial interest since they could be promising platforms for new switching electronic and optical technologies. In this context, we present the first three-dimensional Fe-II Hofmann-type coordination polymer exhibiting SCO properties and luminescence. The complex {Fe-II(bpben)[Au(CN)(2)]}@pyr (bpben = 1,4-bis(4-pyridyl)benzene) functionalized with pyrene (pyr) guests undergoes a cooperative multi-step SCO, which has been investigated by single crystal X-ray diffraction, single crystal UV-Vis absorption spectroscopy, and magnetic and calorimetric measurements. The resulting fluorescence from pyrene and exciplex emissions are controlled by the thermal and light irradiation (LIESST effect) dependence of the high/low-spin state population of Fe-II. Conversely, the SCO can be tracked by monitoring the fluorescence emission. This ON-OFF interplay between SCO and luminescence combined with the amenability of Hofmann-type materials to be processed at the nano-scale may be relevant for the generation of SCO-based sensors, actuators and spintronic devices. | es_ES |
dc.description.sponsorship | This work was supported by the Spanish Ministerio de Economia y Competitividad (MINECO), FEDER (CTQ2013-46275-P and CTQ2016-78341-P), Unidad de Excelencia Maria de Maeztu (MDM-2015-0538), Generalitat Valenciana (PROMETEO/2016/147) and the Swiss National Science Foundation (Project number 200021-169033). | es_ES |
dc.language | Inglés | es_ES |
dc.publisher | The Royal Society of Chemistry | es_ES |
dc.relation.ispartof | Chemical Science | es_ES |
dc.rights | Reconocimiento - No comercial (by-nc) | es_ES |
dc.subject | FE(ABPT)(2)(NCX)(2) X | es_ES |
dc.subject | State | es_ES |
dc.subject | Transition | es_ES |
dc.subject | Complexes | es_ES |
dc.subject | Behavior | es_ES |
dc.subject | Nanocomposite | es_ES |
dc.subject | Hysteresis | es_ES |
dc.subject | Pressure | es_ES |
dc.subject | Emission | es_ES |
dc.subject | Networks | es_ES |
dc.subject.classification | FISICA APLICADA | es_ES |
dc.title | Thermo- and photo-modulation of exciplex fluorescence in a 3D spin crossover Hofmann-type coordination polymer | es_ES |
dc.type | Artículo | es_ES |
dc.identifier.doi | 10.1039/c8sc02677g | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/SNSF//200021_169033/CH/Fundamental studies of boron hydrogen compounds from BH4- to B12H122- and derived compounds and luminescence studies on energy transfer in rare earth containing phosphors/ | |
dc.relation.projectID | info:eu-repo/grantAgreement/MINECO//CTQ2013-46275-P/ES/SENSORES Y MEMORIAS BASADOS EN MATERIALES BIESTABLES CON TRANSICION DE ESPIN/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/GVA//PROMETEO2016%2F147/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/MINECO//CTQ2016-78341-P/ES/MATERIALES SPIN CROSSOVER BIESTABLES: DE LAS PROPIEDADES MACROSCOPICAS A LA ESPINTRONICA MOLECULAR/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/MINECO//MDM-2015-0538/ES/INSTITUTO DE CIENCIA MOLECULAR/ | es_ES |
dc.rights.accessRights | Abierto | es_ES |
dc.contributor.affiliation | Universitat Politècnica de València. Departamento de Física Aplicada - Departament de Física Aplicada | es_ES |
dc.description.bibliographicCitation | Delgado, T.; Meneses-Sánchez, M.; Piñeiro-López, L.; Bartual-Murgui, C.; Muñoz Roca, MDC.; Real, J. (2018). Thermo- and photo-modulation of exciplex fluorescence in a 3D spin crossover Hofmann-type coordination polymer. Chemical Science. 9(44):8446-8452. https://doi.org/10.1039/c8sc02677g | es_ES |
dc.description.accrualMethod | S | es_ES |
dc.relation.publisherversion | https://doi.org/10.1039/c8sc02677g | es_ES |
dc.description.upvformatpinicio | 8446 | es_ES |
dc.description.upvformatpfin | 8452 | es_ES |
dc.type.version | info:eu-repo/semantics/publishedVersion | es_ES |
dc.description.volume | 9 | es_ES |
dc.description.issue | 44 | es_ES |
dc.identifier.pmid | 30542594 | es_ES |
dc.identifier.pmcid | PMC6247521 | es_ES |
dc.relation.pasarela | S\373561 | es_ES |
dc.contributor.funder | Generalitat Valenciana | es_ES |
dc.contributor.funder | Swiss National Science Foundation | es_ES |
dc.contributor.funder | European Regional Development Fund | es_ES |
dc.contributor.funder | Ministerio de Economía y Competitividad | es_ES |
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