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Laser Heating Tunability by Off-Resonant Irradiation of Gold Nanoparticles

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Laser Heating Tunability by Off-Resonant Irradiation of Gold Nanoparticles

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dc.contributor.author Hormeño, S. es_ES
dc.contributor.author Gregorio-Godoy, P. es_ES
dc.contributor.author Pérez-Juste, J. es_ES
dc.contributor.author Liz-Marzán, L.M. es_ES
dc.contributor.author Juárez, B.H. es_ES
dc.contributor.author Arias-Gonzalez, J. R. es_ES
dc.date.accessioned 2020-10-21T03:31:34Z
dc.date.available 2020-10-21T03:31:34Z
dc.date.issued 2014-01-29 es_ES
dc.identifier.issn 1613-6810 es_ES
dc.identifier.uri http://hdl.handle.net/10251/152720
dc.description "This is the peer reviewed version of the following article: Hormeño, Silvia, Paula Gregorio-Godoy, Jorge Pérez-Juste, Luis M. Liz-Marzán, Beatriz H. Juárez, and J. Ricardo Arias-Gonzalez. 2013. Laser Heating Tunability by Off-Resonant Irradiation of Gold Nanoparticles. Small 10 (2). Wiley: 376 84. doi:10.1002/smll.201301912, which has been published in final form at https://doi.org/10.1002/smll.201301912. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Self-Archiving." es_ES
dc.description.abstract [EN] Temperature changes in the vicinity of a single absorptive nanostructure caused by local heating have strong implications in technologies such as integrated electronics or biomedicine. Herein, the temperature changes in the vicinity of a single optically trapped spherical Au nanoparticle encapsulated in a thermo¿responsive poly(N¿isopropylacrylamide) shell (Au@pNIPAM) are studied in detail. Individual beads are trapped in a counter¿propagating optical tweezers setup at various laser powers, which allows the overall particle size to be tuned through the phase transition of the thermo¿responsive shell. The experimentally obtained sizes measured at different irradiation powers are compared with average size values obtained by dynamic light scattering (DLS) from an ensemble of beads at different temperatures. The size range and the tendency to shrink upon increasing the laser power in the optical trap or by increasing the temperature for DLS agree with reasonable accuracy for both approaches. Discrepancies are evaluated by means of simple models accounting for variations in the thermal conductivity of the polymer, the viscosity of the aqueous solution and the absorption cross section of the coated Au nanoparticle. These results show that these parameters must be taken into account when considering local laser heating experiments in aqueous solution at the nanoscale. Analysis of the stability of the Au@pNIPAM particles in the trap is also theoretically carried out for different particle sizes. es_ES
dc.description.sponsorship This work has been partially supported by Comunidad de Madrid through NANOBIOMAGNET S2009-MAT-1726 and the Spanish Ministry of Science and Innovation through RYC-2007-01709, RYC-2007-01765 and MAT-2009-13488. P. G-G. acknowledges a Research Initiation Grant at IMDEA Nanociencia. The authors thank Dr. Reinhold Wannemacher for fruitful discussions. es_ES
dc.language Inglés es_ES
dc.publisher John Wiley & Sons es_ES
dc.relation.ispartof Small es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject Optical tweezers es_ES
dc.subject Thermoresponsive pNIPAM es_ES
dc.subject Au nanoparticles es_ES
dc.subject Hydrodynamic size es_ES
dc.subject Laser heating es_ES
dc.subject.classification FISICA APLICADA es_ES
dc.title Laser Heating Tunability by Off-Resonant Irradiation of Gold Nanoparticles es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1002/smll.201301912 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MEC//RYC-2007-01765/ES/RYC-2007-01765/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MEC//RYC-2007-01709/ES/RYC-2007-01709/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MICINN//MAT2009-13488/ES/Crecimiento Y Caracterizacion De Nuevos Nanomateriales Basados En El Autoensamblado De Puntos Cuanticos Y Nanotubos De Carbono Sobre Superficies Solidas/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/CAM//S2009%2FMAT-1726/ES/Fundamentos y aplicaciones de moléculas, nanopartículas y nanoestructuras magnéticas: de la espintrónica a la biomedicina/ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Física Aplicada - Departament de Física Aplicada es_ES
dc.description.bibliographicCitation Hormeño, S.; Gregorio-Godoy, P.; Pérez-Juste, J.; Liz-Marzán, L.; Juárez, B.; Arias-Gonzalez, JR. (2014). Laser Heating Tunability by Off-Resonant Irradiation of Gold Nanoparticles. Small. 10(2):376-384. https://doi.org/10.1002/smll.201301912 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1002/smll.201301912 es_ES
dc.description.upvformatpinicio 376 es_ES
dc.description.upvformatpfin 384 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 10 es_ES
dc.description.issue 2 es_ES
dc.identifier.pmid 24106098 es_ES
dc.relation.pasarela S\408016 es_ES
dc.contributor.funder Comunidad de Madrid es_ES
dc.contributor.funder Ministerio de Ciencia e Innovación es_ES
dc.contributor.funder Ministerio de Educación y Ciencia es_ES
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