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Enhancement of the processing window and performance of polyamide 1010/bio-based high-density polyethylene blends by melt mixing with natural additives

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Enhancement of the processing window and performance of polyamide 1010/bio-based high-density polyethylene blends by melt mixing with natural additives

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dc.contributor.author Quiles-Carrillo, Luis es_ES
dc.contributor.author Montanes, Nestor es_ES
dc.contributor.author Fombuena, Vicent es_ES
dc.contributor.author Balart, Rafael es_ES
dc.contributor.author Torres-Giner, Sergio es_ES
dc.date.accessioned 2021-02-16T04:32:12Z
dc.date.available 2021-02-16T04:32:12Z
dc.date.issued 2020-01 es_ES
dc.identifier.issn 0959-8103 es_ES
dc.identifier.uri http://hdl.handle.net/10251/161383
dc.description.abstract [EN] This work reports the enhancement of the processing window and the mechanical and thermal properties of biopolymer blends of polyamide 1010 (PA1010) and bio-based high-density polyethylene (bio-HDPE) at 70/30 (wt/wt) achieved by means of natural additives. The overall performance of the binary blend melt-mixed without additives was poor due to both the relatively low thermal stability of bio-HDPE at the processing temperatures of PA1010, that is, 210¿240 ºC, and the lack or poor miscibility between the two biopolymers. Gallic acid (GA), a natural phenolic compound, was added at 0.8 parts per hundred resin (phr) of biopolymer blend to enhance the thermal stability of the green polyolefin and therefore enlarge the processing window of the binary blend. Maleinized linseed oil (MLO), a multi-functionalized vegetable oil, was then incorporated at 5 phr to compatibilize the biopolymers and its performance was also compared with that of a conventional petroleum-derived copolymer, namely, poly(ethylene-co-acrylic acid) (PE-co-AA). The resultant biopolymer blends showed a remarkable enhancement in the thermal stability and also improved toughness when both natural additives were combined. This work can potentially serve as a sound base study for the mechanical recycling of similar blends based on bio-based but non-biodegradable polymers. es_ES
dc.description.sponsorship This research was funded by the Spanish Ministry of Science, Innovation, and Universities (MICIU) project numbers MAT2017-84909-C2-2-R and AGL2015-63855-C2-1-R. LQ-C and ST-G are recipients of an FPU grant (FPU15/03812) from the Spanish Ministry of Education, Culture, and Sports (MECD) and a Juan de la Cierva-Incorporacion contract (IJCI-2016-29675) from MICIU, respectively. The microscopy services at Universitat Politecnica de Valencia (UPV) are acknowledged for their help in collecting and analysing FESEM images. es_ES
dc.language Inglés es_ES
dc.publisher John Wiley & Sons es_ES
dc.relation.ispartof Polymer International es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject PA1010 es_ES
dc.subject Green polyethylene es_ES
dc.subject Thermal stability es_ES
dc.subject Mechanical properties es_ES
dc.subject Secondary recycling es_ES
dc.subject.classification INGENIERIA QUIMICA es_ES
dc.subject.classification CIENCIA DE LOS MATERIALES E INGENIERIA METALURGICA es_ES
dc.subject.classification TECNOLOGIA DE ALIMENTOS es_ES
dc.title Enhancement of the processing window and performance of polyamide 1010/bio-based high-density polyethylene blends by melt mixing with natural additives es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1002/pi.5919 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//IJCI-2016-29675/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//AGL2015-63855-C2-1-R/ES/DESARROLLO DE UN CONCEPTO DE ENVASE MULTICAPA ALIMENTARIO DE ALTA BARRERA Y CON CARACTER ACTIVO Y BIOACTIVO DERIVADO DE SUBPRODUCTOS ALIMENTARIOS/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MECD//FPU15%2F03812/ES/FPU15%2F03812/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/MAT2017-84909-C2-2-R/ES/PROCESADO Y OPTIMIZACION DE MATERIALES AVANZADOS DERIVADOS DE ESTRUCTURAS PROTEICAS Y COMPONENTES LIGNOCELULOSICOS/ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Ingeniería Química y Nuclear - Departament d'Enginyeria Química i Nuclear es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Ingeniería Mecánica y de Materiales - Departament d'Enginyeria Mecànica i de Materials es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto Universitario de Ingeniería de Alimentos para el Desarrollo - Institut Universitari d'Enginyeria d'Aliments per al Desenvolupament es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto de Tecnología de Materiales - Institut de Tecnologia de Materials es_ES
dc.description.bibliographicCitation Quiles-Carrillo, L.; Montanes, N.; Fombuena, V.; Balart, R.; Torres-Giner, S. (2020). Enhancement of the processing window and performance of polyamide 1010/bio-based high-density polyethylene blends by melt mixing with natural additives. Polymer International. 69(1):61-71. https://doi.org/10.1002/pi.5919 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1002/pi.5919 es_ES
dc.description.upvformatpinicio 61 es_ES
dc.description.upvformatpfin 71 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 69 es_ES
dc.description.issue 1 es_ES
dc.relation.pasarela S\397232 es_ES
dc.contributor.funder Agencia Estatal de Investigación es_ES
dc.contributor.funder Ministerio de Educación, Cultura y Deporte es_ES
dc.contributor.funder Ministerio de Economía y Competitividad es_ES
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