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Solid polymer electrolytes based on lithium bis(trifluoromethanesulfonyl)imide/poly(vinylidene fluoride -co-hexafluoropropylene) for safer rechargeable lithium-ion batteries

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Solid polymer electrolytes based on lithium bis(trifluoromethanesulfonyl)imide/poly(vinylidene fluoride -co-hexafluoropropylene) for safer rechargeable lithium-ion batteries

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dc.contributor.author Gonçalves, R. es_ES
dc.contributor.author Miranda, D. es_ES
dc.contributor.author Almeida, A. M. es_ES
dc.contributor.author Silva, M. M. es_ES
dc.contributor.author Meseguer Dueñas, José María es_ES
dc.contributor.author Gómez Ribelles, José Luís es_ES
dc.contributor.author Lanceros-Méndez, S. es_ES
dc.contributor.author Costa, C. M. es_ES
dc.date.accessioned 2021-03-01T08:08:59Z
dc.date.available 2021-03-01T08:08:59Z
dc.date.issued 2019-09 es_ES
dc.identifier.issn 2214-9937 es_ES
dc.identifier.uri http://hdl.handle.net/10251/162579
dc.description.abstract [EN] The increasing use of electronic portable systems and the consequent energy demand, leads to the need to improve energy storage systems. According to that and due to safety issues, high-performance non-flammable electrolytes and solid polymer electrolytes (SPE) are needed. SPE containing different amounts of lithium bis(trifluoromethanesulfonyl) imide (LiTFSI) into a poly(vinylidene fluoride-co-hexafluoropropylene), PVDF-HFP, polymer matrix have been prepared by solvent casting. The addition of LiTFSI into PVDF-HFP allows to tailor thermal, mechanical and electrical properties of the composite. In particular, the ionic conductivity of the composites increases with LiTFSI content, the best ionic conductivities of 0.0011 mS/cmat 25 degrees C and 0.23 mS/cmat 90 degrees C were obtained for the PVDF-HFP/LiTFSI composites with 80 wt % of LiTFSI. This solid electrolyte allows the fabrication of Li metallic/SPE/C-LiFePO4 half-cells with a discharge capacity of 51.2 mAh/ g at C/20. Further, theoretical simulations show that the discharge capacity value depends on the lithium concentration and percentage of free ions and is independent of the solid polymer electrolyte thickness. On the other hand, the voltage plateau depends on the SPE thickness. Thus, a solid electrolyte is presented for the next generation of safer solid-state batteries. es_ES
dc.description.sponsorship The authors thank the FCT (Fundacao para a Ciencia e Tecnologia) for financial support under the framework of Strategic Funding grants UID/FIS/04650/2013, UID/EEA/04436/2013 and UID/QUI/0686/2016; and project no. PTDC/FIS-MAC/28157/2017. The authors also thank the FCT for financial support under grant SFRH/BPD/112547/2015 (C.M.C.). Financial support from the Basque Government Industry Department under the ELKARTEK and HAZITEK programs is also acknowledged. JMMD and JLGR acknowledge funding by the Spanish Ministry of Economy and Competitiveness (MINECO) through the project MAT2016-76039-C4-1 and 3-R (including the FEDER financial support) CIBER-BBN is an initiative funded by the VI National R&D&i Plan 2008-2011, Iniciativa Ingenio 2010, Consolider Program, CIBER Actions and financed by the Instituto de Salud Carlos III with assistance fromthe European Regional Development Fund. es_ES
dc.language Inglés es_ES
dc.publisher Elsevier es_ES
dc.relation.ispartof Sustainable Materials and Technologies es_ES
dc.rights Reconocimiento - No comercial - Sin obra derivada (by-nc-nd) es_ES
dc.subject Solid polymer electrolyte es_ES
dc.subject PVDF-HFP es_ES
dc.subject LiTFSI es_ES
dc.subject Composites es_ES
dc.subject Simulations es_ES
dc.subject Li-ion batteries es_ES
dc.subject.classification FISICA APLICADA es_ES
dc.subject.classification MAQUINAS Y MOTORES TERMICOS es_ES
dc.title Solid polymer electrolytes based on lithium bis(trifluoromethanesulfonyl)imide/poly(vinylidene fluoride -co-hexafluoropropylene) for safer rechargeable lithium-ion batteries es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1016/j.susmat.2019.e00104 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/FCT/SFRH/FCT%2FSFRH%2FBPD%2F112547%2F2015/PT/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/FCT/5876/147325/PT/Microelectromechanical Systems Research Unit/
dc.relation.projectID info:eu-repo/grantAgreement/FCT//UID%2FQUI%2F0686%2F2016/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/FCT/5876/147414/PT/Physics Center of Minho and Porto Universities/
dc.relation.projectID info:eu-repo/grantAgreement/FCT//PTDC%2FFIS-MAC%2F28157%2F2017/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//MAT2016-76039-C4-3-R/ES/UNA NUEVA GENERACION DE MATERIALES ELECTROACTIVOS Y BIOREACTORES PARA INGENIERIA DE TEJIDO MUSCULAR/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//MAT2016-76039-C4-1-R/ES/BIOMATERIALES PIEZOELECTRICOS PARA LA DIFERENCIACION CELULAR EN INTERFASES CELULA-MATERIAL ELECTRICAMENTE ACTIVAS/ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Física Aplicada - Departament de Física Aplicada es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Termodinámica Aplicada - Departament de Termodinàmica Aplicada es_ES
dc.description.bibliographicCitation Gonçalves, R.; Miranda, D.; Almeida, AM.; Silva, MM.; Meseguer Dueñas, JM.; Gómez Ribelles, JL.; Lanceros-Méndez, S.... (2019). Solid polymer electrolytes based on lithium bis(trifluoromethanesulfonyl)imide/poly(vinylidene fluoride -co-hexafluoropropylene) for safer rechargeable lithium-ion batteries. Sustainable Materials and Technologies. 21:1-11. https://doi.org/10.1016/j.susmat.2019.e00104 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1016/j.susmat.2019.e00104 es_ES
dc.description.upvformatpinicio 1 es_ES
dc.description.upvformatpfin 11 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 21 es_ES
dc.relation.pasarela S\404552 es_ES
dc.contributor.funder Instituto de Salud Carlos III es_ES
dc.contributor.funder Gobierno Vasco/Eusko Jaurlaritza es_ES
dc.contributor.funder European Regional Development Fund es_ES
dc.contributor.funder Ministerio de Economía y Competitividad es_ES
dc.contributor.funder Fundação para a Ciência e a Tecnologia, Portugal es_ES
dc.contributor.funder Centro de Investigación Biomédica en Red en Bioingeniería, Biomateriales y Nanomedicina es_ES
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