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dc.contributor.author | Pavanello, Alice | es_ES |
dc.contributor.author | Blasco-Brusola, Alejandro | es_ES |
dc.contributor.author | Johnston, Peter F. | es_ES |
dc.contributor.author | Miranda Alonso, Miguel Ángel | es_ES |
dc.contributor.author | Marín García, Mª Luisa | es_ES |
dc.date.accessioned | 2021-03-25T04:31:25Z | |
dc.date.available | 2021-03-25T04:31:25Z | |
dc.date.issued | 2020-07 | es_ES |
dc.identifier.uri | http://hdl.handle.net/10251/164215 | |
dc.description.abstract | [EN] Four silver phosphate-based materials were successfully synthesized, characterized, and evaluated, together with TiO2, in the photodegradation of synthetic dyes (tartrazine, Orange II, rhodamine, and Brilliant Blue FCF) under two irradiation sources centered at 420 and 450 nm. Scanning Electron Microscopy (SEM) images showed different topologies of the synthesized materials, whereas diffuse reflectance spectra demonstrated that they display absorption up to 500 nm. Degradation experiments were performed in parallel with the silver materials and TiO2. Upon irradiation centered at 420 nm, the abatement of the dyes was slightly more efficient in the case of TiO2-except for Orange II. Nevertheless, upon irradiation centered at 450 nm, TiO(2)demonstrated complete inefficiency and silver phosphates accomplished the complete abatement of the dyes-except for Brilliant Blue FCF. A careful analysis of the achieved degradation of dyes revealed that the main reaction mechanism involves electron transfer to the photogenerated holes in the valence band of silver photocatalysts, together with the direct excitation of dyes and the subsequent formation of reactive species. The performance of TiO(2)was only comparable at the shorter wavelength when hydroxyl radicals could be formed; however, it could not compete under irradiation at 450 nm since the formed superoxide anion is not as reactive as hydroxyl radicals. | es_ES |
dc.description.sponsorship | This research was funded by Spanish Government (Grant SEV-2016-0683), Generalitat Valenciana (Prometeo Program) and H2020/Marie Sklodowska-Curie Actions under the AQUAlity project (Reference: 765860). The authors would like to acknowledge H2020/Marie Sk¿odowska-Curie Actions under the AQUAlity project (Reference: 765860). Consellería d¿Educació, Investigació, Cultura i Esport (PROMETEO/2017/075 and GRISOLÍAP/2017/005) is gratefully acknowledged. | es_ES |
dc.language | Inglés | es_ES |
dc.publisher | MDPI AG | es_ES |
dc.relation.ispartof | Catalysts | es_ES |
dc.rights | Reconocimiento (by) | es_ES |
dc.subject | Conduction band | es_ES |
dc.subject | Hole | es_ES |
dc.subject | Hydroxyl radical | es_ES |
dc.subject | Mechanism | es_ES |
dc.subject | Superoxide anion | es_ES |
dc.subject | Titanium dioxide | es_ES |
dc.subject | Valence band | es_ES |
dc.subject.classification | QUIMICA ORGANICA | es_ES |
dc.title | Enhanced Photodegradation of Synthetic Dyes Mediated by Ag3PO4-Based Semiconductors under Visible Light Irradiation | es_ES |
dc.type | Artículo | es_ES |
dc.identifier.doi | 10.3390/catal10070774 | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/EC/H2020/765860/EU/Interdisciplinar cross-sectoral approach to effectively address the removal of contaminants of emerging concern from water/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/GVA//GRISOLIAP%2F2017%2F005/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/MINECO//SEV-2016-0683/ | es_ES |
dc.relation.projectID | info:eu-repo/grantAgreement/GVA//PROMETEO%2F2017%2F075/ES/Reacciones fotoquímicas de biomoléculas/ | es_ES |
dc.rights.accessRights | Abierto | es_ES |
dc.contributor.affiliation | Universitat Politècnica de València. Departamento de Química - Departament de Química | es_ES |
dc.description.bibliographicCitation | Pavanello, A.; Blasco-Brusola, A.; Johnston, PF.; Miranda Alonso, MÁ.; Marín García, ML. (2020). Enhanced Photodegradation of Synthetic Dyes Mediated by Ag3PO4-Based Semiconductors under Visible Light Irradiation. Catalysts. 10(7):1-17. https://doi.org/10.3390/catal10070774 | es_ES |
dc.description.accrualMethod | S | es_ES |
dc.relation.publisherversion | https://doi.org/10.3390/catal10070774 | es_ES |
dc.description.upvformatpinicio | 1 | es_ES |
dc.description.upvformatpfin | 17 | es_ES |
dc.type.version | info:eu-repo/semantics/publishedVersion | es_ES |
dc.description.volume | 10 | es_ES |
dc.description.issue | 7 | es_ES |
dc.identifier.eissn | 2073-4344 | es_ES |
dc.relation.pasarela | S\416310 | es_ES |
dc.contributor.funder | European Commission | es_ES |
dc.contributor.funder | Generalitat Valenciana | es_ES |
dc.contributor.funder | Ministerio de Economía y Competitividad | es_ES |
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