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Synthesis, post-synthetic modification and stability of a 2D styryl ammonium lead iodide hybrid material

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Synthesis, post-synthetic modification and stability of a 2D styryl ammonium lead iodide hybrid material

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dc.contributor.author Peng, Yong es_ES
dc.contributor.author Albero-Sancho, Josep es_ES
dc.contributor.author García Gómez, Hermenegildo es_ES
dc.date.accessioned 2021-04-28T03:31:28Z
dc.date.available 2021-04-28T03:31:28Z
dc.date.issued 2020-01-14 es_ES
dc.identifier.issn 1477-9226 es_ES
dc.identifier.uri http://hdl.handle.net/10251/165714
dc.description.abstract [EN] A new hybrid lead iodide material (HP1) having 4-vinylphenylene ammonium as the organic cation has been prepared. The structural formula based on chemical analysis of HP1 corresponds to PbI2.5(4-styrylammonium)(0.5). The crystallinity of HP1 was confirmed by powder X-ray diffraction and high resolution transmission electron microscopy. The presence of the styryl ammonium moiety in HP1 allows post-synthetic modification by radical copolymerization with styrene to obtain the HP2 material with higher hydrophobicity. Stability tests reveal that both HP1 and HP2 show hydrogen evolution in the dark, indicating about 0.6% partial decomposition of the hybrid material. This hydrogen evolution increases by a factor of 3 when HP1 and HP2 are exposed to visible light. X-ray photoelectron spectroscopy analysis shows an increase of NH2 groups and a decrease of NH3+ units suggesting that the origin of hydrogen evolution is the deprotonation of ammonium ions. es_ES
dc.description.sponsorship Financial support from the Spanish Ministry of Economy and Competitiveness (Severo Ochoa SEV2016, and RTI2018-890237-CO2-R1) and the Generalitat Valenciana (Prometeo 2017/083) is gratefully acknowledged. Yong Peng also thanks the Universitat Politecnica de Valencia for a predoctoral scholarship. es_ES
dc.language Inglés es_ES
dc.publisher The Royal Society of Chemistry es_ES
dc.relation.ispartof Dalton Transactions es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject.classification QUIMICA ORGANICA es_ES
dc.title Synthesis, post-synthetic modification and stability of a 2D styryl ammonium lead iodide hybrid material es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1039/C9DT04285G es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//SEV-2016-0683/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//RTI2018-890237-CO2-R1 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/GVA//PROMETEO%2F2017%2F083/ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Química - Departament de Química es_ES
dc.description.bibliographicCitation Peng, Y.; Albero-Sancho, J.; García Gómez, H. (2020). Synthesis, post-synthetic modification and stability of a 2D styryl ammonium lead iodide hybrid material. Dalton Transactions. 49(2):395-403. https://doi.org/10.1039/C9DT04285G es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1039/C9DT04285G es_ES
dc.description.upvformatpinicio 395 es_ES
dc.description.upvformatpfin 403 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 49 es_ES
dc.description.issue 2 es_ES
dc.relation.pasarela S\398878 es_ES
dc.contributor.funder Generalitat Valenciana es_ES
dc.contributor.funder Ministerio de Economía y Competitividad es_ES
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