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A Lamellar MWW Zeolite With Silicon and Niobium Oxide Pillars: A Catalyst for the Oxidation of Volatile Organic Compounds

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A Lamellar MWW Zeolite With Silicon and Niobium Oxide Pillars: A Catalyst for the Oxidation of Volatile Organic Compounds

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dc.contributor.author Schwanke, Anderson Joel es_ES
dc.contributor.author Balzer, Rosana es_ES
dc.contributor.author Lopes, Christian Wittee es_ES
dc.contributor.author Meira, Debora Motta es_ES
dc.contributor.author DÍAZ MORALES, URBANO MANUEL es_ES
dc.contributor.author Corma Canós, Avelino es_ES
dc.contributor.author Pergher, Sibele es_ES
dc.date.accessioned 2021-04-28T03:31:39Z
dc.date.available 2021-04-28T03:31:39Z
dc.date.issued 2020-08-17 es_ES
dc.identifier.issn 0947-6539 es_ES
dc.identifier.uri http://hdl.handle.net/10251/165715
dc.description This is the peer reviewed version of the following article: A. J. Schwanke, R. Balzer, C. Wittee Lopes, D. Motta Meira, U. Díaz, A. Corma, S. Pergher, Chem. Eur. J. 2020, 26, 10459, which has been published in final form at https://doi.org/10.1002/chem.202000862. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Self-Archiving. es_ES
dc.description.abstract [EN] In this work, an MWW-type zeolite with pillars containing silicon and niobium oxide was synthesized to obtain a hierarchical zeolite. The effect of niobium insertion in the pillaring process was determined by combining a controllable acidity and accessibility in the final material. All pillared materials had niobium occupying framework positions in pillars and extra-framework positions. The pillared material, Pil-Nb-4.5 with 4.5 wt % niobium, did not compromise the mesoporosity formed by pillaring, while the increase of niobium in the structure gradually decreased the mesoporosity and ordering of lamellar stacking. The morphology of the pillared zeolites and the niobium content were found to directly affect the catalytic activity. Specifically, we report on the activity of the MWW-type zeolites with niobium catalyzing the gas-phase oxidation of volatile organic compounds (VOCs), which is an important reaction for clean environmental. All produced MWW-type zeolites with niobium were catalytically active, even at low temperatures and low niobium loading, and provided excellent conversion efficiencies. es_ES
dc.description.sponsorship A.J.S. thanks the CordenacAo de Aperfeicoamento de Pessoal de Nivel Superior-Brasil (CAPES)-Finance Code 001, the PDSE program (process number 99999.004779/2014-02) and the prof. Claudio Radtke from the PPGQ-UFRGS for the XPS analyses. C.W.L. is grateful to INOMAT/CAPES for a postdoctoral fellowship. U.D. thanks the funding by the Spanish Government (MAT2017-82288-C2-1-P). es_ES
dc.language Inglés es_ES
dc.publisher John Wiley & Sons es_ES
dc.relation.ispartof Chemistry - A European Journal es_ES
dc.rights Reserva de todos los derechos es_ES
dc.subject Layered compounds es_ES
dc.subject MCM-36 es_ES
dc.subject Niobium es_ES
dc.subject Oxidation es_ES
dc.subject Zeolite es_ES
dc.subject.classification QUIMICA ORGANICA es_ES
dc.title A Lamellar MWW Zeolite With Silicon and Niobium Oxide Pillars: A Catalyst for the Oxidation of Volatile Organic Compounds es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1002/chem.202000862 es_ES
dc.relation.projectID info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/MAT2017-82288-C2-1-P/ES/MATERIALES HIBRIDOS MULTIFUNCIONALES BASADOS EN NANO-UNIDADES ESTRUCTURALES ACTIVAS/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/CAPES//001/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/CAPES//99999.004779%2F2014-02/ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Química - Departament de Química es_ES
dc.description.bibliographicCitation Schwanke, AJ.; Balzer, R.; Lopes, CW.; Meira, DM.; Díaz Morales, UM.; Corma Canós, A.; Pergher, S. (2020). A Lamellar MWW Zeolite With Silicon and Niobium Oxide Pillars: A Catalyst for the Oxidation of Volatile Organic Compounds. Chemistry - A European Journal. 26(46):1-12. https://doi.org/10.1002/chem.202000862 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1002/chem.202000862 es_ES
dc.description.upvformatpinicio 1 es_ES
dc.description.upvformatpfin 12 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 26 es_ES
dc.description.issue 46 es_ES
dc.identifier.pmid 32427389 es_ES
dc.relation.pasarela S\434007 es_ES
dc.contributor.funder Coordenaçao de Aperfeiçoamento de Pessoal de Nível Superior, Brasil es_ES
dc.contributor.funder Agencia Estatal de Investigación es_ES
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