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Direct synthesis of the organic and Ge free Al containing BOG zeolite (ITQ-47) and its application for transformation of biomass derived molecules

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Direct synthesis of the organic and Ge free Al containing BOG zeolite (ITQ-47) and its application for transformation of biomass derived molecules

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dc.contributor.author Huang, Qintong es_ES
dc.contributor.author Chen, Ningyue es_ES
dc.contributor.author Liu, Lichen es_ES
dc.contributor.author Arias-Carrascal, Karen Sulay es_ES
dc.contributor.author Iborra Chornet, Sara es_ES
dc.contributor.author Yi, Xianfeng es_ES
dc.contributor.author Ma, Chao es_ES
dc.contributor.author Lianf, Weichi es_ES
dc.contributor.author Zheng, Anmin es_ES
dc.contributor.author Zhang, Chuanqi es_ES
dc.contributor.author Hu, Jibo es_ES
dc.contributor.author Cai, Zilin es_ES
dc.contributor.author Liu, Yi es_ES
dc.contributor.author Jiang, Jiuxing es_ES
dc.contributor.author Corma Canós, Avelino es_ES
dc.date.accessioned 2021-04-29T03:32:05Z
dc.date.available 2021-04-29T03:32:05Z
dc.date.issued 2020-11-28 es_ES
dc.identifier.issn 2041-6520 es_ES
dc.identifier.uri http://hdl.handle.net/10251/165766
dc.description.abstract [EN] Aluminosilicate boggsite (Si/Al-BOG) has been hydrothermally synthesized without adding org. structure-directing agents (OSDAs) in the synthesis gel using the borosilicogermanium ITQ-47 (Si/B-ITQ-47) zeolite as seeds. The introduction of the costly and environmentally less benign phosphazene org. structure-directing agent is not required to grow the zeolite. Physicochem. characterization expts. show that Si/Al-BOG has good crystallinity, high surface area, tetrahedral Al3+ species, and acid sites. In order to test the catalytic performance of the zeolite, the synthesis of L,L-lactide from L-lactic acid was performed. Si/Al-BOG exhibits 88.2% conversion of L-lactic acid and 83.8% L,L-lactide selectivity, which are better than those of other zeolites studied up to now. es_ES
dc.description.sponsorship This work was supported by the National Natural Science Foundation of China 21971259 and 91645112, The Natural Science Foundation of Hubei Province of China (2014CFA043), and the Key Research Program of Frontier Sciences, CAS (No. QYZDB-SSW-SLH026). The European Union is also acknowledged by ERC-AdG-2014-671093 SynCatMatch, and the Spanish Government through "Severo Ochoa" (SEV-2016-0683, MINECO). Q. H. acknowledges the International Program Fund for doctoral students, Sun Yat-sen University, for scholarships in Spain. es_ES
dc.language Inglés es_ES
dc.publisher The Royal Society of Chemistry es_ES
dc.relation.ispartof Chemical Science es_ES
dc.rights Reconocimiento - No comercial (by-nc) es_ES
dc.subject.classification QUIMICA ORGANICA es_ES
dc.title Direct synthesis of the organic and Ge free Al containing BOG zeolite (ITQ-47) and its application for transformation of biomass derived molecules es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.1039/d0sc04044d es_ES
dc.relation.projectID info:eu-repo/grantAgreement/EC/H2020/671093/EU/MATching zeolite SYNthesis with CATalytic activity/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/MINECO//SEV-2016-0683/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/NSFC//21971259/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/NSFC//91645112/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/Natural Science Foundation of Hubei Province//2014CFA043/ es_ES
dc.relation.projectID info:eu-repo/grantAgreement/CAS//QYZDB-SSW-SLH026/ es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Química - Departament de Química es_ES
dc.description.bibliographicCitation Huang, Q.; Chen, N.; Liu, L.; Arias-Carrascal, KS.; Iborra Chornet, S.; Yi, X.; Ma, C.... (2020). Direct synthesis of the organic and Ge free Al containing BOG zeolite (ITQ-47) and its application for transformation of biomass derived molecules. Chemical Science. 11(44):12103-12108. https://doi.org/10.1039/d0sc04044d es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.1039/d0sc04044d es_ES
dc.description.upvformatpinicio 12103 es_ES
dc.description.upvformatpfin 12108 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 11 es_ES
dc.description.issue 44 es_ES
dc.relation.pasarela S\433150 es_ES
dc.contributor.funder European Commission es_ES
dc.contributor.funder Sun Yat-sen University es_ES
dc.contributor.funder Chinese Academy of Sciences es_ES
dc.contributor.funder National Natural Science Foundation of China es_ES
dc.contributor.funder Natural Science Foundation of Hubei Province es_ES
dc.contributor.funder Ministerio de Economía y Competitividad es_ES
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