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Identification of Foulants on Polyethersulfone Membranes Used to Remove Colloids and Dissolved Matter from Paper Mill Treated Effluent

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Identification of Foulants on Polyethersulfone Membranes Used to Remove Colloids and Dissolved Matter from Paper Mill Treated Effluent

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dc.contributor.author Sousa, Mayko Rannany S. es_ES
dc.contributor.author Lora-García, Jaime es_ES
dc.contributor.author López Pérez, Maria Fernanda es_ES
dc.contributor.author Heran, Marc es_ES
dc.date.accessioned 2021-05-25T03:32:12Z
dc.date.available 2021-05-25T03:32:12Z
dc.date.issued 2020-02 es_ES
dc.identifier.issn 2073-4441 es_ES
dc.identifier.uri http://hdl.handle.net/10251/166738
dc.description.abstract [EN] In this study, membrane fouling caused by paperboard mill treated effluent (PMTE) was investigated based on a dead-end ultrafiltration (UF) pilot-scale study. The membranes employed were commercial hydrophobic UF membranes made of polyethersulfone (PES) with a molecular weight cut-off of 10 kDa, 50 kDa, and 100 kDa. Membrane fouling mechanism during dead-end filtration, chemical analysis, field emission scanning electron microscopy (FESEM), energy-dispersive spectrophotometry (EDS), attenuated total reflection-Fourier transform infrared (ATR-FTIR) spectroscopy and 3D fluorescence excitation emission matrix (3DEEM) analysis were applied to understand which fraction of the dissolved and colloidal substances (DCS) caused the membrane fouling. The results indicated that the phenomenon controlling fouling mechanism tended to be cake layer formation (R-2 >= 0.98) for all membranes tested. The 3DEEM results indicate that the majority of the organic foulants with fluorescence characteristics on the membrane were colloidal proteins (protein-like substances I+II) and macromolecular proteins (soluble microbial products, SMP-like substances). In addition, polysaccharide (cellulosic species), fatty and resin acid substances were identified on the fouled membrane by the ATR-FTIR analysis and play an important role in membrane fouling. In addition, the FESEM and EDS analyses indicate that the presence of inorganic foulants on the membrane surfaces, such as metal ions and especially Ca2+, can accelerate membrane fouling, whereas Mg and Si are linked to reversible fouling. es_ES
dc.language Inglés es_ES
dc.publisher MDPI AG es_ES
dc.relation.ispartof Water es_ES
dc.rights Reconocimiento (by) es_ES
dc.subject Ultrafiltration es_ES
dc.subject Paper mill effluent es_ES
dc.subject Membrane fouling es_ES
dc.subject Foulants identification es_ES
dc.subject.classification INGENIERIA QUIMICA es_ES
dc.title Identification of Foulants on Polyethersulfone Membranes Used to Remove Colloids and Dissolved Matter from Paper Mill Treated Effluent es_ES
dc.type Artículo es_ES
dc.identifier.doi 10.3390/w12020365 es_ES
dc.rights.accessRights Abierto es_ES
dc.contributor.affiliation Universitat Politècnica de València. Departamento de Ingeniería Química y Nuclear - Departament d'Enginyeria Química i Nuclear es_ES
dc.description.bibliographicCitation Sousa, MRS.; Lora-García, J.; López Pérez, MF.; Heran, M. (2020). Identification of Foulants on Polyethersulfone Membranes Used to Remove Colloids and Dissolved Matter from Paper Mill Treated Effluent. Water. 12(2):1-27. https://doi.org/10.3390/w12020365 es_ES
dc.description.accrualMethod S es_ES
dc.relation.publisherversion https://doi.org/10.3390/w12020365 es_ES
dc.description.upvformatpinicio 1 es_ES
dc.description.upvformatpfin 27 es_ES
dc.type.version info:eu-repo/semantics/publishedVersion es_ES
dc.description.volume 12 es_ES
dc.description.issue 2 es_ES
dc.relation.pasarela S\402423 es_ES
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