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Selective room-temperature transformation of methane to C1 Oxygenates by deep UV Photolysis over zeolites

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Selective room-temperature transformation of methane to C1 Oxygenates by deep UV Photolysis over zeolites

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Sastre Calabuig, F.; Fornes Seguí, V.; Corma Canós, A.; García Gómez, H. (2011). Selective room-temperature transformation of methane to C1 Oxygenates by deep UV Photolysis over zeolites. Journal of the American Chemical Society. 133(43):17257-17261. doi:10.1021/ja204559z

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Título: Selective room-temperature transformation of methane to C1 Oxygenates by deep UV Photolysis over zeolites
Autor:
Entidad UPV: Universitat Politècnica de València. Departamento de Química - Departament de Química
Fecha difusión:
Resumen:
Methane can directly be transformed into liquid C 1 oxygenated products with selectivities above 95% at 13% conversion by deep UV photocatalysis, in the presence of H 2O and air. Pure silica zeolites, and more specifically, ...[+]
Palabras clave: Amorphous silica , Beta zeolite , Confined space , Deep uv , Homolytic cleavage , Methyl radical , Micropores , Oxygenated products , Pure silica zeolites , Room temperature , Silanol groups , Solid surface , Surface hydroxyl groups , Carbon monoxide , Energy utilization , Methane , Photocatalysis , Photolysis , Reaction intermediates , Silica , Silicate minerals , Synthesis (chemical) , Synthesis gas , Zeolites , Liquid methane , C1 oxygenate , Oxygen derivative , Silanol , Silicate , Unclassified drug , Zeolite , Article , Energy consumption , Micropore filter , Oxygenation , Ultraviolet radiation , Oxygen , Temperature , Ultraviolet Rays
Derechos de uso: Cerrado
Fuente:
Journal of the American Chemical Society. (issn: 0002-7863 )
DOI: 10.1021/ja204559z
Editorial:
American Chemical Society
Versión del editor: dx.doi.org/10.1021/ja204559z
Agradecimientos:
Financial support by the Spanish Ministry of Science and Innovation (MICINN Grants CTQ-2009-0585 and CONSOLIDER INGENIO MULTICAT) is gratefully acknowledged.
Tipo: Artículo

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