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Activity of ceria and ceria-supported gold nanoparticles for the carbamoylation of aliphatic amines by dimethyl carbonate

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Activity of ceria and ceria-supported gold nanoparticles for the carbamoylation of aliphatic amines by dimethyl carbonate

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Juárez Marín, R.; Corma Canós, A.; García Gómez, H. (2011). Activity of ceria and ceria-supported gold nanoparticles for the carbamoylation of aliphatic amines by dimethyl carbonate. Pure and Applied Chemistry. 84(3):685-694. doi:10.1351/PAC-CON-11-06-06

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Título: Activity of ceria and ceria-supported gold nanoparticles for the carbamoylation of aliphatic amines by dimethyl carbonate
Autor:
Entidad UPV: Universitat Politècnica de València. Departamento de Química - Departament de Química
Universitat Politècnica de València. Instituto Universitario Mixto de Tecnología Química - Institut Universitari Mixt de Tecnologia Química
Fecha difusión:
Resumen:
Aliphatic amines react sluggishly with dimethyl carbonate (DMC) to give a mixture of N-methylation and carbamoylation. Nanoparticulated ceria as catalyst increases, in general, conversion and selectivity toward carbamoylation. ...[+]
Palabras clave: Carbamoylation , Catalysts , Gold , Gold nanoparticles , Green chemistry , Phosgene-free synthesis of isocyanates
Derechos de uso: Reconocimiento - Sin obra derivada - No comercial (by-nd-nc)
Fuente:
Pure and Applied Chemistry. (issn: 0033-4545 ) (eissn: 1365-3075 )
DOI: 10.1351/PAC-CON-11-06-06
Editorial:
International Union of Pure and Applied Chemistry
Versión del editor: http://dx.doi.org/10.1351/PAC-CON-11-06-06
Agradecimientos:
Financial support by the Spanish Ministry of Science and Innovation (Consolider 2010-CSD2009-0050 and CTQ2009-11586) is gratefully acknowledged. R.J. thanks the Spanish Ministry of Education for a postgraduate scholarship.[+]
Tipo: Artículo

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