- -

'From the mole to the molecule': ruthenium catalyzed nitroarene reduction studied with 'bench', high-throughput and single molecule fluorescence techniques

RiuNet: Institutional repository of the Polithecnic University of Valencia

Share/Send to

Cited by

Statistics

'From the mole to the molecule': ruthenium catalyzed nitroarene reduction studied with 'bench', high-throughput and single molecule fluorescence techniques

Show full item record

Carrillo, AI.; Stamplecoskie, KG.; Marín García, ML.; Scaiano, JC. (2014). 'From the mole to the molecule': ruthenium catalyzed nitroarene reduction studied with 'bench', high-throughput and single molecule fluorescence techniques. Catalysis Science and Technology. 4(7):1989-1996. doi:10.1039/c4cy00018h

Por favor, use este identificador para citar o enlazar este ítem: http://hdl.handle.net/10251/61429

Files in this item

Item Metadata

Title: 'From the mole to the molecule': ruthenium catalyzed nitroarene reduction studied with 'bench', high-throughput and single molecule fluorescence techniques
Author:
UPV Unit: Universitat Politècnica de València. Departamento de Química - Departament de Química
Universitat Politècnica de València. Instituto Universitario Mixto Tecnológico de Informática - Institut Universitari Mixt Tecnològic d'Informàtica
Issued date:
Abstract:
Single molecule fluorescence microscopy techniques are used to complement conventional catalysis and high-throughput experiments in order to gain a complete picture of a model reaction. In these experiments a model nitroarene ...[+]
Subjects: HETEROGENEOUS CATALYSTS , GOLD NANOPARTICLES , COUPLING REACTIONS , REACTIVITY , COMPLEXES , ARYLATION , DYNAMICS
Copyrigths: Reserva de todos los derechos
Source:
Catalysis Science and Technology. (issn: 2044-4753 ) (eissn: 2044-4761 )
DOI: 10.1039/c4cy00018h
Publisher:
Royal Society of Chemistry
Publisher version: http://dx.doi.org/10.1039/c4cy00018h
Thanks:
Thanks are due to the Natural Sciences and Engineering Council of Canada and the Canadian Foundation for Innovation for generous support. M. L. Marin thanks the Universitat Politecnica de Valencia (Programa de Apoyo a la ...[+]
Type: Artículo

References

Stauffer, S. R., & Hartwig, J. F. (2003). Fluorescence Resonance Energy Transfer (FRET) as a High-Throughput Assay for Coupling Reactions. Arylation of Amines as a Case Study. Journal of the American Chemical Society, 125(23), 6977-6985. doi:10.1021/ja034161p

McNally, A., Prier, C. K., & MacMillan, D. W. C. (2011). Discovery of an  -Amino C-H Arylation Reaction Using the Strategy of Accelerated Serendipity. Science, 334(6059), 1114-1117. doi:10.1126/science.1213920

Roeffaers, M. â J., Deâ Cremer, G., Libeert, J., Ameloot, R., Dedecker, P., Bons, A.-J., … Hofkens, J. (2009). Super-Resolution Reactivity Mapping of Nanostructured Catalyst Particles. Angewandte Chemie International Edition, 48(49), 9285-9289. doi:10.1002/anie.200904944 [+]
Stauffer, S. R., & Hartwig, J. F. (2003). Fluorescence Resonance Energy Transfer (FRET) as a High-Throughput Assay for Coupling Reactions. Arylation of Amines as a Case Study. Journal of the American Chemical Society, 125(23), 6977-6985. doi:10.1021/ja034161p

McNally, A., Prier, C. K., & MacMillan, D. W. C. (2011). Discovery of an  -Amino C-H Arylation Reaction Using the Strategy of Accelerated Serendipity. Science, 334(6059), 1114-1117. doi:10.1126/science.1213920

Roeffaers, M. â J., Deâ Cremer, G., Libeert, J., Ameloot, R., Dedecker, P., Bons, A.-J., … Hofkens, J. (2009). Super-Resolution Reactivity Mapping of Nanostructured Catalyst Particles. Angewandte Chemie International Edition, 48(49), 9285-9289. doi:10.1002/anie.200904944

Roeffaers, M. B. J., Hofkens, J., De Cremer, G., De Schryver, F. C., Jacobs, P. A., De Vos, D. E., & Sels, B. F. (2007). Fluorescence microscopy: Bridging the phase gap in catalysis. Catalysis Today, 126(1-2), 44-53. doi:10.1016/j.cattod.2007.03.007

Tachikawa, T., & Majima, T. (2012). Single-Molecule, Single-Particle Approaches for Exploring the Structure and Kinetics of Nanocatalysts. Langmuir, 28(24), 8933-8943. doi:10.1021/la300177h

Zhou, X., Xu, W., Liu, G., Panda, D., & Chen, P. (2010). Size-Dependent Catalytic Activity and Dynamics of Gold Nanoparticles at the Single-Molecule Level. Journal of the American Chemical Society, 132(1), 138-146. doi:10.1021/ja904307n

Wee, T.-L. (Erika), Schmidt, L. C., & Scaiano, J. C. (2012). Photooxidation of 9-Anthraldehyde Catalyzed by Gold Nanoparticles: Solution and Single Nanoparticle Studies Using Fluorescence Lifetime Imaging. The Journal of Physical Chemistry C, 116(45), 24373-24379. doi:10.1021/jp308956y

Carrillo, A. I., Schmidt, L. C., Marín, M. L., & Scaiano, J. C. (2014). Mild synthesis of mesoporous silica supported ruthenium nanoparticles as heterogeneous catalysts in oxidative Wittig coupling reactions. Catal. Sci. Technol., 4(2), 435-440. doi:10.1039/c3cy00773a

Del Pozo, C., Corma, A., Iglesias, M., & Sánchez, F. (2011). Recyclable mesoporous silica-supported chiral ruthenium-(NHC)NN-pincer catalysts for asymmetric reactions. Green Chemistry, 13(9), 2471. doi:10.1039/c1gc15412e

HAJEK, J. (2003). Ruthenium-modified MCM-41 mesoporous molecular sieve and Y zeolite catalysts for selective hydrogenation of cinnamaldehyde. Applied Catalysis A: General, 251(2), 385-396. doi:10.1016/s0926-860x(03)00345-4

Prier, C. K., Rankic, D. A., & MacMillan, D. W. C. (2013). Visible Light Photoredox Catalysis with Transition Metal Complexes: Applications in Organic Synthesis. Chemical Reviews, 113(7), 5322-5363. doi:10.1021/cr300503r

Szadkowska, A., Samojłowicz, C., & Grela, K. (2011). Enhancement of ruthenium-catalyzed olefin metathesis reactions: Searching for new catalyst or new reaction conditions? Pure and Applied Chemistry, 83(3), 553-563. doi:10.1351/pac-con-10-09-10

Lara, P., Philippot, K., & Chaudret, B. (2012). Organometallic Ruthenium Nanoparticles: A Comparative Study of the Influence of the Stabilizer on their Characteristics and Reactivity. ChemCatChem, 5(1), 28-45. doi:10.1002/cctc.201200666

R. H. Grubbs , Handbook of Metathesis, Wiley-VCH, Weinheim, 2003

Jansat, S., Picurelli, D., Pelzer, K., Philippot, K., Gómez, M., Muller, G., … Chaudret, B. (2006). Synthesis, characterization and catalytic reactivity of ruthenium nanoparticles stabilized by chiral N-donor ligands. New J. Chem., 30(1), 115-122. doi:10.1039/b509378c

Salas, G., Campbell, P. S., Santini, C. C., Philippot, K., Costa Gomes, M. F., & Pádua, A. A. H. (2012). Ligand effect on the catalytic activity of ruthenium nanoparticles in ionic liquids. Dalton Transactions, 41(45), 13919. doi:10.1039/c2dt31644g

Davies, I. W., Matty, L., Hughes, D. L., & Reider, P. J. (2001). Are Heterogeneous Catalysts Precursors to Homogeneous Catalysts? Journal of the American Chemical Society, 123(41), 10139-10140. doi:10.1021/ja016877v

Montoya, L. A., & Pluth, M. D. (2012). Selective turn-on fluorescent probes for imaging hydrogen sulfide in living cells. Chemical Communications, 48(39), 4767. doi:10.1039/c2cc30730h

Larsen, J. W., Freund, M., Kim, K. Y., Sidovar, M., & Stuart, J. L. (2000). Mechanism of the carbon catalyzed reduction of nitrobenzene by hydrazine. Carbon, 38(5), 655-661. doi:10.1016/s0008-6223(99)00155-4

Al-Soufi, W., Reija, B., Novo, M., Felekyan, S., Kühnemuth, R., & Seidel, C. A. M. (2005). Fluorescence Correlation Spectroscopy, a Tool to Investigate Supramolecular Dynamics:  Inclusion Complexes of Pyronines with Cyclodextrin. Journal of the American Chemical Society, 127(24), 8775-8784. doi:10.1021/ja0508976

Witham, C. A., Huang, W., Tsung, C.-K., Kuhn, J. N., Somorjai, G. A., & Toste, F. D. (2009). Converting homogeneous to heterogeneous in electrophilic catalysis using monodisperse metal nanoparticles. Nature Chemistry, 2(1), 36-41. doi:10.1038/nchem.468

Nishina, Y., Miyata, J., Kawai, R., & Gotoh, K. (2012). Recyclable Pd–graphene catalyst: mechanistic insights into heterogeneous and homogeneous catalysis. RSC Advances, 2(25), 9380. doi:10.1039/c2ra21185h

Nørskov, J. K., Bligaard, T., Rossmeisl, J., & Christensen, C. H. (2009). Towards the computational design of solid catalysts. Nature Chemistry, 1(1), 37-46. doi:10.1038/nchem.121

[-]

This item appears in the following Collection(s)

Show full item record