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[+]
Burgos-Asperilla, L., Darder, M., Aranda, P., Vázquez, L., Vázquez, M., & Ruiz-Hitzky, E. (2007). Novel magnetic organic–inorganic nanostructured materials. Journal of Materials Chemistry, 17(40), 4233. doi:10.1039/b706011d
Gomez-Romero, P. (2001). Hybrid Organic-Inorganic Materials—In Search of Synergic Activity. Advanced Materials, 13(3), 163-174. doi:10.1002/1521-4095(200102)13:3<163::aid-adma163>3.0.co;2-u
Fernandez-Saavedra, R., Aranda, P., Carrado, K., Sandi, G., Seifert, S., & Ruiz-Hitzky, E. (2009). Template Synthesis of Nanostructured Carbonaceous Materials for Application in Electrochemical Devices. Current Nanoscience, 5(4), 506-513. doi:10.2174/157341309789378168
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Chen, W., Xu, Q., Hu, Y. S., Mai, L. Q., & Zhu, Q. Y. (2002). Effect of modification by poly(ethylene oxide) on the reversibility of insertion/extraction of Li+ ion in V2O5 xerogel films. Journal of Materials Chemistry, 12(6), 1926-1929. doi:10.1039/b203056j
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Chen, W., Mai, L., Qi, Y., & Dai, Y. (2006). One-dimensional nanomaterials of vanadium and molybdenum oxides. Journal of Physics and Chemistry of Solids, 67(5-6), 896-902. doi:10.1016/j.jpcs.2006.01.074
Willinger, M.-G., Neri, G., Rauwel, E., Bonavita, A., Micali, G., & Pinna, N. (2008). Vanadium Oxide Sensing Layer Grown on Carbon Nanotubes by a New Atomic Layer Deposition Process. Nano Letters, 8(12), 4201-4204. doi:10.1021/nl801785b
White, R. J., Budarin, V. L., & Clark, J. H. (2008). Tuneable Mesoporous Materials from α-D-Polysaccharides. ChemSusChem, 1(5), 408-411. doi:10.1002/cssc.200800012
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Hu, B., Wang, K., Wu, L., Yu, S.-H., Antonietti, M., & Titirici, M.-M. (2010). Engineering Carbon Materials from the Hydrothermal Carbonization Process of Biomass. Advanced Materials, 22(7), 813-828. doi:10.1002/adma.200902812
Dujardin, E., Blaseby, M., & Mann, S. (2003). Synthesis of mesoporous silica by sol–gel mineralisation of cellulose nanorod nematic suspensions. Journal of Materials Chemistry, 13(4), 696-699. doi:10.1039/b212689c
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Macquarrie, D. J., & Hardy, J. J. E. (2005). Applications of Functionalized Chitosan in Catalysis†. Industrial & Engineering Chemistry Research, 44(23), 8499-8520. doi:10.1021/ie050007v
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El Kadib, A., Katir, N., Marcotte, N., Molvinger, K., Castel, A., Rivière, P., & Brunel, D. (2009). Nanocomposites from natural templates based on fatty compound-functionalised siloxanes. Journal of Materials Chemistry, 19(33), 6004. doi:10.1039/b906448f
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Molvinger, K., Quignard, F., Brunel, D., Boissière, M., & Devoisselle, J.-M. (2004). Porous Chitosan-Silica Hybrid Microspheres as a Potential Catalyst. Chemistry of Materials, 16(17), 3367-3372. doi:10.1021/cm0353299
Kadib, A. E., Molvinger, K., Guimon, C., Quignard, F., & Brunel, D. (2008). Design of Stable Nanoporous Hybrid Chitosan/Titania as Cooperative Bifunctional Catalysts. Chemistry of Materials, 20(6), 2198-2204. doi:10.1021/cm800080s
Kadib, A. E., Molvinger, K., Bousmina, M., & Brunel, D. (2010). Improving Catalytic Activity by Synergic Effect between Base and Acid Pairs in Hierarchically Porous Chitosan@Titania Nanoreactors. Organic Letters, 12(5), 948-951. doi:10.1021/ol9029319
Kadib, A. E., Molvinger, K., Bousmina, M., & Brunel, D. (2010). Decoration of chitosan microspheres with inorganic oxide clusters: Rational design of hierarchically porous, stable and cooperative acid–base nanoreactors. Journal of Catalysis, 273(2), 147-155. doi:10.1016/j.jcat.2010.05.010
Kadib, A. E., Molvinger, K., Cacciaguerra, T., Bousmina, M., & Brunel, D. (2011). Chitosan templated synthesis of porous metal oxide microspheres with filamentary nanostructures. Microporous and Mesoporous Materials, 142(1), 301-307. doi:10.1016/j.micromeso.2010.12.012
Review:
Mallat, T., & Baiker, A. (2004). Oxidation of Alcohols with Molecular Oxygen on Solid Catalysts. Chemical Reviews, 104(6), 3037-3058. doi:10.1021/cr0200116
De Vos, D. E., Dams, M., Sels, B. F., & Jacobs, P. A. (2002). Ordered Mesoporous and Microporous Molecular Sieves Functionalized with Transition Metal Complexes as Catalysts for Selective Organic Transformations. Chemical Reviews, 102(10), 3615-3640. doi:10.1021/cr010368u
For selected examples see:
Karimi, B., Abedi, S., Clark, J. H., & Budarin, V. (2006). Highly Efficient Aerobic Oxidation of Alcohols Using a Recoverable Catalyst: The Role of Mesoporous Channels of SBA-15 in Stabilizing Palladium Nanoparticles. Angewandte Chemie, 118(29), 4894-4897. doi:10.1002/ange.200504359
Karimi, B., Abedi, S., Clark, J. H., & Budarin, V. (2006). Highly Efficient Aerobic Oxidation of Alcohols Using a Recoverable Catalyst: The Role of Mesoporous Channels of SBA-15 in Stabilizing Palladium Nanoparticles. Angewandte Chemie International Edition, 45(29), 4776-4779. doi:10.1002/anie.200504359
Mori, K., Yamaguchi, K., Hara, T., Mizugaki, T., Ebitani, K., & Kaneda, K. (2002). Controlled Synthesis of Hydroxyapatite-Supported Palladium Complexes as Highly Efficient Heterogeneous Catalysts. Journal of the American Chemical Society, 124(39), 11572-11573. doi:10.1021/ja020444q
Mori, K., Hara, T., Mizugaki, T., Ebitani, K., & Kaneda, K. (2004). Hydroxyapatite-Supported Palladium Nanoclusters: A Highly Active Heterogeneous Catalyst for Selective Oxidation of Alcohols by Use of Molecular Oxygen. Journal of the American Chemical Society, 126(34), 10657-10666. doi:10.1021/ja0488683
Yamaguchi, K., & Mizuno, N. (2002). Angewandte Chemie, 114(23), 4720-4724. doi:10.1002/1521-3757(20021202)114:23<4720::aid-ange4720>3.0.co;2-p
Yamaguchi, K., & Mizuno, N. (2002). Supported Ruthenium Catalyst for the Heterogeneous Oxidation of Alcohols with Molecular Oxygen. Angewandte Chemie International Edition, 41(23), 4538-4542. doi:10.1002/1521-3773(20021202)41:23<4538::aid-anie4538>3.0.co;2-6
Enache, D. I., Edwards, J. K., Landon, P., Solsona-Espriu, B., Carley, A. F., Herzing, A. A., … Hutchings, G. J. (2006). Solvent-Free Oxidation of Primary Alcohols to Aldehydes Using Au-Pd/TiO2 Catalysts. Science, 311(5759), 362-365. doi:10.1126/science.1120560
Abad, A., Concepción, P., Corma, A., & García, H. (2005). A Collaborative Effect between Gold and a Support Induces the Selective Oxidation of Alcohols. Angewandte Chemie, 117(26), 4134-4137. doi:10.1002/ange.200500382
Abad, A., Concepción, P., Corma, A., & García, H. (2005). A Collaborative Effect between Gold and a Support Induces the Selective Oxidation of Alcohols. Angewandte Chemie International Edition, 44(26), 4066-4069. doi:10.1002/anie.200500382
Comotti, M., Della Pina, C., Matarrese, R., & Rossi, M. (2004). The Catalytic Activity of ?Naked? Gold Particles. Angewandte Chemie, 116(43), 5936-5939. doi:10.1002/ange.200460446
Comotti, M., Della Pina, C., Matarrese, R., & Rossi, M. (2004). The Catalytic Activity of ?Naked? Gold Particles. Angewandte Chemie International Edition, 43(43), 5812-5815. doi:10.1002/anie.200460446
HOU, W., DEHM, N., & SCOTT, R. (2008). Alcohol oxidations in aqueous solutions using Au, Pd, and bimetallic AuPd nanoparticle catalysts. Journal of Catalysis, 253(1), 22-27. doi:10.1016/j.jcat.2007.10.025
Miyamura, H., Matsubara, R., Miyazaki, Y., & Kobayashi, S. (2007). Aerobic Oxidation of Alcohols at Room Temperature and Atmospheric Conditions Catalyzed by Reusable Gold Nanoclusters Stabilized by the Benzene Rings of Polystyrene Derivatives. Angewandte Chemie, 119(22), 4229-4232. doi:10.1002/ange.200700080
Miyamura, H., Matsubara, R., Miyazaki, Y., & Kobayashi, S. (2007). Aerobic Oxidation of Alcohols at Room Temperature and Atmospheric Conditions Catalyzed by Reusable Gold Nanoclusters Stabilized by the Benzene Rings of Polystyrene Derivatives. Angewandte Chemie International Edition, 46(22), 4151-4154. doi:10.1002/anie.200700080
Miyamura, H., Matsubara, R., & Kobayashi, S. (2008). Gold–platinum bimetallic clusters for aerobic oxidation of alcohols under ambient conditions. Chemical Communications, (17), 2031. doi:10.1039/b800657a
Chan-Thaw, C. E., Villa, A., Katekomol, P., Su, D., Thomas, A., & Prati, L. (2010). Covalent Triazine Framework as Catalytic Support for Liquid Phase Reaction. Nano Letters, 10(2), 537-541. doi:10.1021/nl904082k
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Karimi, B., Ghoreishi-Nezhad, M., & Clark, J. H. (2005). Selective Oxidation of Sulfides to Sulfoxides Using 30% Hydrogen Peroxide Catalyzed with a Recoverable Silica-Based Tungstate Interphase Catalyst. Organic Letters, 7(4), 625-628. doi:10.1021/ol047635d
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The stability of chitosan under acidic and basic conditions has been discussed in ref. [15a]. Immersion of native chitosan beads in acetic acid (0.1 n) resulted in solubilisation of the gel network.
Barringer, E. A., & Bowen, H. K. (1985). High-purity, monodisperse TiO2 powders by hydrolysis of titanium tetraethoxide. 1. Synthesis and physical properties. Langmuir, 1(4), 414-420. doi:10.1021/la00064a005
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Larionova, J., Salmon, L., Guari, Y., Tokarev, A., Molvinger, K., Molnár, G., & Bousseksou, A. (2008). Towards the Ultimate Size Limit of the Memory Effect in Spin-Crossover Solids. Angewandte Chemie International Edition, 47(43), 8236-8240. doi:10.1002/anie.200802906
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Wan, D., Yuan, S., Li, G. L., Neoh, K. G., & Kang, E. T. (2010). Glucose Biosensor from Covalent Immobilization of Chitosan-Coupled Carbon Nanotubes on Polyaniline-Modified Gold Electrode. ACS Applied Materials & Interfaces, 2(11), 3083-3091. doi:10.1021/am100591t
Muylaert, I., Borgers, M., Bruneel, E., Schaubroeck, J., Verpoort, F., & Van Der Voort, P. (2008). Ultra stable ordered mesoporous phenol/formaldehyde polymers as a heterogeneous support for vanadium oxide. Chemical Communications, (37), 4475. doi:10.1039/b808566h
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Sueoka, S., Mitsudome, T., Mizugaki, T., Jitsukawa, K., & Kaneda, K. (2010). Supported monomeric vanadium catalyst for dehydration of amides to form nitriles. Chemical Communications, 46(43), 8243. doi:10.1039/c0cc02412k
Khatri, P. K., Singh, B., Jain, S. L., Sain, B., & Sinha, A. K. (2011). Cyclotriphosphazene grafted silica: a novel support for immobilizing the oxo-vanadium Schiff base moieties for hydroxylation of benzene. Chem. Commun., 47(5), 1610-1612. doi:10.1039/c0cc01941k
El Kadib, A., Chimenton, R., Sachse, A., Fajula, F., Galarneau, A., & Coq, B. (2009). Functionalized Inorganic Monolithic Microreactors for High Productivity in Fine Chemicals Catalytic Synthesis. Angewandte Chemie, 121(27), 5069-5072. doi:10.1002/ange.200805580
El Kadib, A., Chimenton, R., Sachse, A., Fajula, F., Galarneau, A., & Coq, B. (2009). Functionalized Inorganic Monolithic Microreactors for High Productivity in Fine Chemicals Catalytic Synthesis. Angewandte Chemie International Edition, 48(27), 4969-4972. doi:10.1002/anie.200805580
Aguado, S., Canivet, J., & Farrusseng, D. (2010). Facile shaping of an imidazolate-based MOF on ceramic beads for adsorption and catalytic applications. Chemical Communications, 46(42), 7999. doi:10.1039/c0cc02045a
Sorokin, A. B., Quignard, F., Valentin, R., & Mangematin, S. (2006). Chitosan supported phthalocyanine complexes: Bifunctional catalysts with basic and oxidation active sites. Applied Catalysis A: General, 309(2), 162-168. doi:10.1016/j.apcata.2006.03.060
Guo, C.-C., Huang, G., Zhang, X.-B., & Guo, D.-C. (2003). Catalysis of chitosan-supported iron tetraphenylporphyrin for aerobic oxidation of cyclohexane in absence of reductants and solvents. Applied Catalysis A: General, 247(2), 261-267. doi:10.1016/s0926-860x(03)00108-x
Karimi, B., & Kabiri Esfahani, F. (2009). Gold nanoparticles supported on Cs2CO3 as recyclable catalyst system for selective aerobic oxidation of alcohols at room temperature. Chemical Communications, (37), 5555. doi:10.1039/b908964k
When monitoring the degradation of the materials used in catalysis by thermogravimetric analysis (TGA)/mass spectroscopy no product attributed to the oxidation of the support was observed.
Chitosan has been shown to be effective for adsorption and removal of vanadium tungsten and molybdenum from aqueous solutions:
Qian, S., Wang, H., Huang, G., Mo, S., & Wei, W. (2004). Studies of adsorption properties of crosslinked chitosan for vanadium(V), tungsten(VI). Journal of Applied Polymer Science, 92(3), 1584-1588. doi:10.1002/app.20102
Kufelnicki, A., Lichawska, M. E., & Bodek, K. H. (2009). Interaction of microcrystalline chitosan (MCCh) with Mo(VI) in aqueous solution. Journal of Applied Polymer Science, 114(3), 1619-1625. doi:10.1002/app.30756
Qian, S. H., Xue, A. F., Xiao, M., & Chen, H. (2006). Application of crosslinked chitosan in the analysis of ultratrace Mo(VI). Journal of Applied Polymer Science, 101(1), 432-435. doi:10.1002/app.23251
Navarro, R., Guzmán, J., Saucedo, I., Revilla, J., & Guibal, E. (2003). Recovery of Metal Ions by Chitosan: Sorption Mechanisms and Influence of Metal Speciation. Macromolecular Bioscience, 3(10), 552-561. doi:10.1002/mabi.200300013
Guzmán, J., Saucedo, I., Navarro, R., Revilla, J., & Guibal, E. (2002). Vanadium Interactions with Chitosan: Influence of Polymer Protonation and Metal Speciation. Langmuir, 18(5), 1567-1573. doi:10.1021/la010802n
In some cases the fast re‐deposition of the leached active species back onto the support can result in a misconception about the result. So in the absence of an exhaustive study on this phenomenon the following results have to be carefully interpreted.
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